Identification of the surface species responsible for N2O formation from the chemisorption of NO on Rh/alumina
Newton, Mark A., Dent, Andrew J., Fiddy, Steven G., Jyoti, Bhrat and Evans, John (2007) Identification of the surface species responsible for N2O formation from the chemisorption of NO on Rh/alumina. Physical Chemistry Chemical Physics, 9, (2), 246-249. (doi:10.1039/b613251k).
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Original Publication URL: http://dx.doi.org/10.1039/b613251k
Description/Abstract
Energy dispersive EXAFS (EDE) and diffuse reflectance infrared spectroscopy (DRIFTS) are combined synchronously at high time resolution (17 Hz) to probe how NO(g) reacts with gamma-Al2O3 supported, metallic Rh nanoparticles of an average 11 A diameter; a bent nitrosyl species is considered to be the key to the formation of N2O.
| Item Type: | Article |
|---|---|
| ISSNs: | 1463-9076 (print) |
| Related URLs: | |
| Keywords: | energy loss characterization, rh catalysts, heterogeneous catalysts, rh/al2o3 catalysts, exhaust catalysis, dispersive exafs, ft-ir, co, rh(111), interconversion |
| Subjects: | Q Science > QD Chemistry Q Science > QC Physics |
| Divisions: | University Structure - Pre August 2011 > School of Chemistry |
| Item ID: | 44593 |
| Date Deposited: | 02 Mar 2007 |
| Last Modified: | 01 Jun 2011 11:52 |
| Contributors: | Newton, Mark A. (Author) Dent, Andrew J. (Author) Fiddy, Steven G. (Author) Jyoti, Bhrat (Author) Evans, John (Author) |
| Date: | 2007 |
| Status: | Published |
| Contact Email Address: | je@soton.ac.uk |
| URI: | http://eprints.soton.ac.uk/id/eprint/44593 |
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