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A new family of sulfur-rich ligands based on the dmit system: synthesis and metal complexation of 4-4'-covalently bridged bis(2-thioxo-1,3-dithiol-5-thiolato) units

A new family of sulfur-rich ligands based on the dmit system: synthesis and metal complexation of 4-4'-covalently bridged bis(2-thioxo-1,3-dithiol-5-thiolato) units
A new family of sulfur-rich ligands based on the dmit system: synthesis and metal complexation of 4-4'-covalently bridged bis(2-thioxo-1,3-dithiol-5-thiolato) units
The synthesis of a new series of sulfur-rich ligands is reported. These compounds, which are related to the dmit(2-) (2-thioxo-1,3-dithiol-4,5-dithiolato) structure, comprise two 2-thioxo-1,3-dithiol-5-thiolato units linked by a bridging unit at the 4-position of the heterocycle via a dithioether spacer unit. Complexation reactions have been carried out on a variety of metal centres; dialkyl tin and gold(I) derivatives have been isolated and fully characterised. The X-ray crystal structure of an octahedral Ni(II) complex, involving two coordinating pyridine molecules, is presented.
x-ray structure, crystal-structure, transition, dithiolate, chemistry, nickel, tetrathiafulvalene, superconductor, reactivity, ni(dmit)2
1472-7773
2654-2659
Allen, David W.
4cbcd21b-4bb9-40e8-baa9-27b1b3e5a7b2
Berridge, Rory
6aa42596-b293-4914-a1eb-2a974e7f2ed4
Bricklebank, Neil
6e082c98-a747-4690-bb37-f05f24d621f5
Cerrada, Elena
e16191cb-1aa4-48f2-9015-99bc01c33423
Light, Mark E.
cf57314e-6856-491b-a8d2-2dffc452e161
Hursthouse, Michael B.
57a2ddf9-b1b3-4f38-bfe9-ef2f526388da
Laguna, Mariano
c2c5e52a-e5ff-4ef7-862a-642401a58db7
Moreno, Ana
aa6d46ad-152d-4f6d-b349-e8fabb15e83c
Skabara, Peter J.
7138e414-7d50-41c7-933e-0bccad2fa4cd
Allen, David W.
4cbcd21b-4bb9-40e8-baa9-27b1b3e5a7b2
Berridge, Rory
6aa42596-b293-4914-a1eb-2a974e7f2ed4
Bricklebank, Neil
6e082c98-a747-4690-bb37-f05f24d621f5
Cerrada, Elena
e16191cb-1aa4-48f2-9015-99bc01c33423
Light, Mark E.
cf57314e-6856-491b-a8d2-2dffc452e161
Hursthouse, Michael B.
57a2ddf9-b1b3-4f38-bfe9-ef2f526388da
Laguna, Mariano
c2c5e52a-e5ff-4ef7-862a-642401a58db7
Moreno, Ana
aa6d46ad-152d-4f6d-b349-e8fabb15e83c
Skabara, Peter J.
7138e414-7d50-41c7-933e-0bccad2fa4cd

Allen, David W., Berridge, Rory, Bricklebank, Neil, Cerrada, Elena, Light, Mark E., Hursthouse, Michael B., Laguna, Mariano, Moreno, Ana and Skabara, Peter J. (2002) A new family of sulfur-rich ligands based on the dmit system: synthesis and metal complexation of 4-4'-covalently bridged bis(2-thioxo-1,3-dithiol-5-thiolato) units. Journal of the Chemical Society, Dalton Transactions, (13), 2654-2659. (doi:10.1039/b201615j).

Record type: Article

Abstract

The synthesis of a new series of sulfur-rich ligands is reported. These compounds, which are related to the dmit(2-) (2-thioxo-1,3-dithiol-4,5-dithiolato) structure, comprise two 2-thioxo-1,3-dithiol-5-thiolato units linked by a bridging unit at the 4-position of the heterocycle via a dithioether spacer unit. Complexation reactions have been carried out on a variety of metal centres; dialkyl tin and gold(I) derivatives have been isolated and fully characterised. The X-ray crystal structure of an octahedral Ni(II) complex, involving two coordinating pyridine molecules, is presented.

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Published date: 2002
Keywords: x-ray structure, crystal-structure, transition, dithiolate, chemistry, nickel, tetrathiafulvalene, superconductor, reactivity, ni(dmit)2

Identifiers

Local EPrints ID: 19654
URI: http://eprints.soton.ac.uk/id/eprint/19654
ISSN: 1472-7773
PURE UUID: ed43d60d-3ce9-4ebf-bf76-943ff8adc640
ORCID for Mark E. Light: ORCID iD orcid.org/0000-0002-0585-0843

Catalogue record

Date deposited: 15 Feb 2006
Last modified: 16 Mar 2024 03:04

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Contributors

Author: David W. Allen
Author: Rory Berridge
Author: Neil Bricklebank
Author: Elena Cerrada
Author: Mark E. Light ORCID iD
Author: Mariano Laguna
Author: Ana Moreno
Author: Peter J. Skabara

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