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Solid-phase construction: high efficiency dendrimer synthesis using AB(3) isocyanate-type monomers

Solid-phase construction: high efficiency dendrimer synthesis using AB(3) isocyanate-type monomers
Solid-phase construction: high efficiency dendrimer synthesis using AB(3) isocyanate-type monomers
Solid-phase synthesis is an ideal tool for reactions that require high concentrations and excess reagents and forcing chemical conditions. One such chemistry is that required for dendrimer construction. In this paper the synthesis of a series of symmetrical AB(3) isocyanate-type monomers is reported and used for the preparation of tri-branched dendrimers on the solid-phase. This method not only allows isolable dendrimer but can generate high-loading supports and devices for multivalent presentation.
solid-phase chemistry, dendrimers, high-loading, multivalency, isocyanatehigh-loading resin, peptide-synthesis, beads, chemistry
0040-4020
3945-3953
Lebreton, S.
565a2f7b-c948-4c19-a7d5-704413341ef2
How, S. E.
fd4a1274-c838-4aaf-a5fc-6b024b0bf664
Buchholz, M.
45681423-2037-48c9-be3c-fbe5ad3bf4f8
Yingyongnarongkul, B. E.
ebde2428-8226-4887-992e-daebeb8eeffa
Bradley, M.
078a34d6-96c4-4ce1-9aa1-454d9ee0030d
Lebreton, S.
565a2f7b-c948-4c19-a7d5-704413341ef2
How, S. E.
fd4a1274-c838-4aaf-a5fc-6b024b0bf664
Buchholz, M.
45681423-2037-48c9-be3c-fbe5ad3bf4f8
Yingyongnarongkul, B. E.
ebde2428-8226-4887-992e-daebeb8eeffa
Bradley, M.
078a34d6-96c4-4ce1-9aa1-454d9ee0030d

Lebreton, S., How, S. E., Buchholz, M., Yingyongnarongkul, B. E. and Bradley, M. (2003) Solid-phase construction: high efficiency dendrimer synthesis using AB(3) isocyanate-type monomers. Tetrahedron, 59 (22), 3945-3953. (doi:10.1016/S0040-4020(03)00463-0).

Record type: Article

Abstract

Solid-phase synthesis is an ideal tool for reactions that require high concentrations and excess reagents and forcing chemical conditions. One such chemistry is that required for dendrimer construction. In this paper the synthesis of a series of symmetrical AB(3) isocyanate-type monomers is reported and used for the preparation of tri-branched dendrimers on the solid-phase. This method not only allows isolable dendrimer but can generate high-loading supports and devices for multivalent presentation.

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More information

Published date: 26 May 2003
Keywords: solid-phase chemistry, dendrimers, high-loading, multivalency, isocyanatehigh-loading resin, peptide-synthesis, beads, chemistry

Identifiers

Local EPrints ID: 20008
URI: http://eprints.soton.ac.uk/id/eprint/20008
ISSN: 0040-4020
PURE UUID: 6200e365-d172-4066-9b8d-bcb2d7b0a512

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Date deposited: 17 Feb 2006
Last modified: 15 Mar 2024 06:21

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Contributors

Author: S. Lebreton
Author: S. E. How
Author: M. Buchholz
Author: B. E. Yingyongnarongkul
Author: M. Bradley

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