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Binding of Co3+ and CoCl42- within a pyridine-cored molecular cleft

Binding of Co3+ and CoCl42- within a pyridine-cored molecular cleft
Binding of Co3+ and CoCl42- within a pyridine-cored molecular cleft
When the novel pyridine-2,6-dicarboxylic acid bis[(quinolin-8-ylmethyl)amide] (PDQA) is treated with CoCl2 a 1:1 complex [(PDQAH(2))][(COCl4)-Cl-II] (2), is formed. Treatment of 2 with NaNO2 results in oxidation of the CoCl42- to Co-III affording [(PDQA-H)Co-III(NO2)(2)] (3) whereas under basic conditions a 2:1 (ligand:Co-III) paddle-like structure [Co-III(PDPA-2H)(2)K(H2O)(2)(CH3 OH)(1)](H2O)(2) (1) is obtained.
tetrachlorocobaltate complexation, anion binding, cobalt complexes, pyridine-cored ligands, supramolecular assembliescarboxamido nitrogens, cobalt(iii) complexes, n coordination, iron(iii), copper(ii), ligands, donors, amine, amide, bonds
1061-0278
405-410
Dwyer, A
d9c9a6eb-18e5-401e-af4e-d149f847912a
Grossel, Martin C.
403bf3ff-6364-44e9-ab46-52d84c6f0d56
Horton, Peter N.
154c8930-bfc3-495b-ad4a-8a278d5da3a5
Dwyer, A
d9c9a6eb-18e5-401e-af4e-d149f847912a
Grossel, Martin C.
403bf3ff-6364-44e9-ab46-52d84c6f0d56
Horton, Peter N.
154c8930-bfc3-495b-ad4a-8a278d5da3a5

Dwyer, A, Grossel, Martin C. and Horton, Peter N. (2004) Binding of Co3+ and CoCl42- within a pyridine-cored molecular cleft. Supramolecular Chemistry, 16 (6), 405-410. (doi:10.1080/10610270410001713312).

Record type: Article

Abstract

When the novel pyridine-2,6-dicarboxylic acid bis[(quinolin-8-ylmethyl)amide] (PDQA) is treated with CoCl2 a 1:1 complex [(PDQAH(2))][(COCl4)-Cl-II] (2), is formed. Treatment of 2 with NaNO2 results in oxidation of the CoCl42- to Co-III affording [(PDQA-H)Co-III(NO2)(2)] (3) whereas under basic conditions a 2:1 (ligand:Co-III) paddle-like structure [Co-III(PDPA-2H)(2)K(H2O)(2)(CH3 OH)(1)](H2O)(2) (1) is obtained.

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More information

Published date: 1 September 2004
Keywords: tetrachlorocobaltate complexation, anion binding, cobalt complexes, pyridine-cored ligands, supramolecular assembliescarboxamido nitrogens, cobalt(iii) complexes, n coordination, iron(iii), copper(ii), ligands, donors, amine, amide, bonds

Identifiers

Local EPrints ID: 20188
URI: http://eprints.soton.ac.uk/id/eprint/20188
ISSN: 1061-0278
PURE UUID: 4532d3a7-2acd-4e17-9e23-d46d3af2c8e3
ORCID for Martin C. Grossel: ORCID iD orcid.org/0000-0001-7469-6854
ORCID for Peter N. Horton: ORCID iD orcid.org/0000-0001-8886-2016

Catalogue record

Date deposited: 22 Feb 2006
Last modified: 16 Mar 2024 03:12

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Contributors

Author: A Dwyer
Author: Peter N. Horton ORCID iD

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