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Alkylated organic cages: from porous crystals to neat liquids

Alkylated organic cages: from porous crystals to neat liquids
Alkylated organic cages: from porous crystals to neat liquids
Rigid organic iminospherand cages are rendered meltable by multiple alkylation; below their melting points they can take the form of permanently porous crystals, crystals unstable to desolvation or nonporous glassy solids depending on chain length and branching; melting points as low as 50 degrees C are observed and a fully Newtonian liquid phase is obtained above 80 degrees C. Thin glassy fibres can be drawn out from a molten phase.
1478-6524
2153-2157
Giri, Nicola
73116700-c23c-439e-be0c-660d436409ff
Davidson, Christine E.
9c4e4db7-7b1f-41b5-88b4-4e947c983450
Melaugh, Gavin
ddff8283-a68d-46fc-9fa8-00d3c266f221
Del Pópolo, Mario G.
e2acde08-cdb9-4ce8-99ba-376012debd74
Jones, James T. A.
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Hasell, Tom
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Cooper, Andrew I.
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Horton, Peter N.
154c8930-bfc3-495b-ad4a-8a278d5da3a5
Hursthouse, Michael B.
57a2ddf9-b1b3-4f38-bfe9-ef2f526388da
James, Stuart L.
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Giri, Nicola
73116700-c23c-439e-be0c-660d436409ff
Davidson, Christine E.
9c4e4db7-7b1f-41b5-88b4-4e947c983450
Melaugh, Gavin
ddff8283-a68d-46fc-9fa8-00d3c266f221
Del Pópolo, Mario G.
e2acde08-cdb9-4ce8-99ba-376012debd74
Jones, James T. A.
ff1f5fb6-a4e3-432c-8113-eba7d35d0c64
Hasell, Tom
6c8f5286-f4e2-456e-a3cd-dcfd3d164e52
Cooper, Andrew I.
95618a3b-7f3f-4731-a0d4-0a7b7ce07302
Horton, Peter N.
154c8930-bfc3-495b-ad4a-8a278d5da3a5
Hursthouse, Michael B.
57a2ddf9-b1b3-4f38-bfe9-ef2f526388da
James, Stuart L.
64b3fff6-707c-4523-823b-e4890ed07b18

Giri, Nicola, Davidson, Christine E., Melaugh, Gavin, Del Pópolo, Mario G., Jones, James T. A., Hasell, Tom, Cooper, Andrew I., Horton, Peter N., Hursthouse, Michael B. and James, Stuart L. (2012) Alkylated organic cages: from porous crystals to neat liquids. Chemical Science, 3 (6), 2153-2157. (doi:10.1039/c2sc01007k).

Record type: Article

Abstract

Rigid organic iminospherand cages are rendered meltable by multiple alkylation; below their melting points they can take the form of permanently porous crystals, crystals unstable to desolvation or nonporous glassy solids depending on chain length and branching; melting points as low as 50 degrees C are observed and a fully Newtonian liquid phase is obtained above 80 degrees C. Thin glassy fibres can be drawn out from a molten phase.

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More information

Published date: 5 April 2012
Organisations: Organic Chemistry: Synthesis, Catalysis and Flow

Identifiers

Local EPrints ID: 347313
URI: http://eprints.soton.ac.uk/id/eprint/347313
ISSN: 1478-6524
PURE UUID: 0d9b946f-097c-4fe8-ba04-4748bad9c4f5
ORCID for Peter N. Horton: ORCID iD orcid.org/0000-0001-8886-2016

Catalogue record

Date deposited: 18 Jan 2013 11:31
Last modified: 15 Mar 2024 03:04

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Contributors

Author: Nicola Giri
Author: Christine E. Davidson
Author: Gavin Melaugh
Author: Mario G. Del Pópolo
Author: James T. A. Jones
Author: Tom Hasell
Author: Andrew I. Cooper
Author: Peter N. Horton ORCID iD
Author: Stuart L. James

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