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Probing the structure and dynamics of molecular clusters using rotational wave packets

Probing the structure and dynamics of molecular clusters using rotational wave packets
Probing the structure and dynamics of molecular clusters using rotational wave packets
Rotational wavepackets of the weakly bound C2H2-He complex have been created using impulsive alignment. The coherent rotational dynamics were monitored for 600 ps enabling extraction of a frequency spectrum showing multiple rotational energy levels up to J = 4. The spectrum has been combined with ab initio calculations to show that the complex has a highly delocalised structure and is bound only by ca. 7 cm
043004/1 to 043004/5
Galinis, G.
67c37798-31c6-4355-985a-b7387e15fb97
Cacho, C.
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Chapman, R.T.
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Ellis, A.M.
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Lewerenz, M.
3c533752-7c1f-4c97-a541-ea4cef34b60d
Mendoza Luna, L.G.
579943ab-9795-4aac-9cb8-d1b1e13497cb
Minns, R.S.
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Mladenovic, M.
0bd6677c-5267-44b9-8b2c-a29b109fbbad
Rouzee, A.
a643168d-4856-4839-8fa3-b66d54c4e035
Springate, E.
740a0cbc-7be5-4c9c-ac28-4d0370b10e2f
Turcu, I.C.E.
6090557e-f0c5-482d-a5c7-b75af0d080c8
Watkins, M.J.
686243cf-6008-4564-83bc-9aede50f8a94
von Haeften, K.
1751d78e-0637-4fef-be50-9691d2ca6278
Galinis, G.
67c37798-31c6-4355-985a-b7387e15fb97
Cacho, C.
3b41ac4c-1dab-466f-8542-15aded608555
Chapman, R.T.
e6cd4194-ec2e-43af-8b66-9b03f2ba13f7
Ellis, A.M.
f634ee53-b614-4a28-8827-2c59e7087fce
Lewerenz, M.
3c533752-7c1f-4c97-a541-ea4cef34b60d
Mendoza Luna, L.G.
579943ab-9795-4aac-9cb8-d1b1e13497cb
Minns, R.S.
85280db4-c5a6-4a4c-82fe-75693c6a6045
Mladenovic, M.
0bd6677c-5267-44b9-8b2c-a29b109fbbad
Rouzee, A.
a643168d-4856-4839-8fa3-b66d54c4e035
Springate, E.
740a0cbc-7be5-4c9c-ac28-4d0370b10e2f
Turcu, I.C.E.
6090557e-f0c5-482d-a5c7-b75af0d080c8
Watkins, M.J.
686243cf-6008-4564-83bc-9aede50f8a94
von Haeften, K.
1751d78e-0637-4fef-be50-9691d2ca6278

Galinis, G., Cacho, C. and Chapman, R.T. et al. (2014) Probing the structure and dynamics of molecular clusters using rotational wave packets. Physical Review Letters, 113 (4), 043004/1 to 043004/5, [43004]. (doi:10.1103/PhysRevLett.113.043004).

Record type: Article

Abstract

Rotational wavepackets of the weakly bound C2H2-He complex have been created using impulsive alignment. The coherent rotational dynamics were monitored for 600 ps enabling extraction of a frequency spectrum showing multiple rotational energy levels up to J = 4. The spectrum has been combined with ab initio calculations to show that the complex has a highly delocalised structure and is bound only by ca. 7 cm

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e-pub ahead of print date: 24 July 2014
Published date: 24 July 2014
Organisations: Chemistry
Learn more about Chemistry research

Identifiers

Local EPrints ID: 367107
URI: http://eprints.soton.ac.uk/id/eprint/367107
DOI: doi:10.1103/PhysRevLett.113.043004
PURE UUID: 7394ea6e-4d15-4894-8d67-02c34bc3cc23
ORCID for R.S. Minns: ORCID iD orcid.org/0000-0001-6775-2977

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Date deposited: 18 Aug 2014 11:42
Last modified: 15 Mar 2024 03:40

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Contributors

Author: G. Galinis
Author: C. Cacho
Author: R.T. Chapman
Author: A.M. Ellis
Author: M. Lewerenz
Author: L.G. Mendoza Luna
Author: R.S. Minns ORCID iD
Author: M. Mladenovic
Author: A. Rouzee
Author: E. Springate
Author: I.C.E. Turcu
Author: M.J. Watkins
Author: K. von Haeften

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