Active template synthesis of rotaxanes and molecular shuttles with switchable dynamics by four-component PdII-promoted michael additions
Active template synthesis of rotaxanes and molecular shuttles with switchable dynamics by four-component PdII-promoted michael additions
Rotaxanes and molecular shuttles are prepared in up to 99?% yield by successive PdII-promoted 1,4-conjugate additions in a one-pot four-component assembly process. This process represents the first active template reaction in which the template motif is retained in the interlocked product.
3381-3384
Goldup, Stephen M.
0a93eedd-98bb-42c1-a963-e2815665e937
Leigh, David A.
826353b6-267f-44cd-a7e7-adf0c34f66c9
Lusby, Paul J.
7edd6163-af61-4425-83ef-bf48d9c9b094
McBurney, Roy T.
200683de-6158-4a21-8d22-68adc26f0e59
Slawin, Alexandra M. Z.
015022ad-00f0-4639-9b31-14b1bd0c234d
20 March 2008
Goldup, Stephen M.
0a93eedd-98bb-42c1-a963-e2815665e937
Leigh, David A.
826353b6-267f-44cd-a7e7-adf0c34f66c9
Lusby, Paul J.
7edd6163-af61-4425-83ef-bf48d9c9b094
McBurney, Roy T.
200683de-6158-4a21-8d22-68adc26f0e59
Slawin, Alexandra M. Z.
015022ad-00f0-4639-9b31-14b1bd0c234d
Goldup, Stephen M., Leigh, David A., Lusby, Paul J., McBurney, Roy T. and Slawin, Alexandra M. Z.
(2008)
Active template synthesis of rotaxanes and molecular shuttles with switchable dynamics by four-component PdII-promoted michael additions.
Angewandte Chemie International Edition, 47 (18), .
(doi:10.1002/anie.200705859).
(PMID:18357597)
Abstract
Rotaxanes and molecular shuttles are prepared in up to 99?% yield by successive PdII-promoted 1,4-conjugate additions in a one-pot four-component assembly process. This process represents the first active template reaction in which the template motif is retained in the interlocked product.
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Published date: 20 March 2008
Organisations:
Organic Chemistry: Synthesis, Catalysis and Flow
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Local EPrints ID: 370664
URI: http://eprints.soton.ac.uk/id/eprint/370664
ISSN: 1433-7851
PURE UUID: b40d3251-5082-4568-9886-efd9e22df4fe
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Date deposited: 03 Nov 2014 13:54
Last modified: 14 Mar 2024 18:20
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Contributors
Author:
David A. Leigh
Author:
Paul J. Lusby
Author:
Roy T. McBurney
Author:
Alexandra M. Z. Slawin
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