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Magnetic MOF microreactors for recyclable size-selective biocatalysis

Magnetic MOF microreactors for recyclable size-selective biocatalysis
Magnetic MOF microreactors for recyclable size-selective biocatalysis
In this contribution we report a synthetic strategy for the encapsulation of functional biomolecules within MOF-based microcapsules. We employ an agarose hydrogel droplet Pickering-stabilised by UiO-66 and magnetite nanoparticles as a template around which to deposit a hierarchically structured ZIF-8 shell. The resulting microcapsules are robust, highly microporous and readily attracted to a magnet, where the hydrogel core provides a facile means to encapsulate enzymes for recyclable size-selective biocatalysis
1478-6524
1938-1943
Huo, Jia
962a200d-5811-424f-b7af-9f98e9c9ae47
Aguilera-Sigalat, Jordi
56421714-a157-49d4-90fc-31b34a148e85
El-Hankari, Samir
553903b7-2f34-4dcd-bd0a-cb0014eb4139
Bradshaw, Darren
7677b11e-1961-447e-b9ba-4847a74bd4dd
Huo, Jia
962a200d-5811-424f-b7af-9f98e9c9ae47
Aguilera-Sigalat, Jordi
56421714-a157-49d4-90fc-31b34a148e85
El-Hankari, Samir
553903b7-2f34-4dcd-bd0a-cb0014eb4139
Bradshaw, Darren
7677b11e-1961-447e-b9ba-4847a74bd4dd

Huo, Jia, Aguilera-Sigalat, Jordi, El-Hankari, Samir and Bradshaw, Darren (2015) Magnetic MOF microreactors for recyclable size-selective biocatalysis. Chemical Science, 6 (3), 1938-1943. (doi:10.1039/C4SC03367A).

Record type: Article

Abstract

In this contribution we report a synthetic strategy for the encapsulation of functional biomolecules within MOF-based microcapsules. We employ an agarose hydrogel droplet Pickering-stabilised by UiO-66 and magnetite nanoparticles as a template around which to deposit a hierarchically structured ZIF-8 shell. The resulting microcapsules are robust, highly microporous and readily attracted to a magnet, where the hydrogel core provides a facile means to encapsulate enzymes for recyclable size-selective biocatalysis

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Accepted/In Press date: 17 December 2014
e-pub ahead of print date: 17 December 2014
Published date: 1 March 2015
Organisations: Chemistry, Organic Chemistry: SCF

Identifiers

Local EPrints ID: 384102
URI: http://eprints.soton.ac.uk/id/eprint/384102
ISSN: 1478-6524
PURE UUID: 0d3b3496-0db8-4388-88e1-197d64b1492f
ORCID for Darren Bradshaw: ORCID iD orcid.org/0000-0001-5258-6224

Catalogue record

Date deposited: 04 Dec 2015 14:40
Last modified: 15 Sep 2021 01:58

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