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The application of flow dispersion models to the FM01-lC laboratory filter-press reactor

Trinidad, P., Ponce de León, C.A. and Walsh, F.C. (2006) The application of flow dispersion models to the FM01-lC laboratory filter-press reactor Electrochimica Acta, 52, (2), pp. 604-613. (doi:10.1016/j.electacta.2006.05.040).

Record type: Article

Abstract

The flow distribution in the rectangular channel of a laboratory filter-press electrochemical reactor was evaluated using three flow models namely (a) axial dispersion, (b) sum of two phases and (c) fast and stagnant zones. In the case of the axial dispersion model, several methods have been used to calculate the Peclet number,; the moment method, the non-linear least squares and the Laplace transform technique. Several boundary conditions, involving different physical and experimental assumptions of the flow were used to solve the partial differential equation that describes the flow behaviour. A total of nine expressions to examine flow dispersion has been used. The comparison of experimental and predicted response signals was made by evaluating the root mean squared error. A data fit in real time has been found to be a better choice as solutions based on the evaluation of moments are prone to error due the overweight of the signal at long times. Data fitting in the Laplace plane is very accurate but it does not guarantee a good fit in real time. Models based on the sum of a fast and a slow or stagnant phase resulted in solutions having very low values of the extension of the slow and stagnant phases, the assumption of a single phase with some degree of dispersion was considered more appropriate.

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More information

Submitted date: 22 December 2005
Published date: 25 October 2006
Keywords: axial dispersion, channel flow, electrochemical reactor, filter-press cell, flow dispersion models, parallel plate geometry, sum of two phases, turbulence
Organisations: Engineering Mats & Surface Engineerg Gp

Identifiers

Local EPrints ID: 39317
URI: http://eprints.soton.ac.uk/id/eprint/39317
ISSN: 0013-4686
PURE UUID: 4e38b90b-1ee3-4257-a161-b0cf0733c031

Catalogue record

Date deposited: 27 Jun 2006
Last modified: 17 Jul 2017 15:37

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