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Tetranuclear Zn2Ln2 coordination clusters as catalysts in the Petasis borono-Mannich multicomponent reaction

Tetranuclear Zn2Ln2 coordination clusters as catalysts in the Petasis borono-Mannich multicomponent reaction
Tetranuclear Zn2Ln2 coordination clusters as catalysts in the Petasis borono-Mannich multicomponent reaction
We report herein for the first time the efficiency of heteronuclear Zn/Ln coordination clusters (CCs) as catalysts for the multicomponent Mannich-type condensation that involves amines, aldehydes and boronic acids, known as the Petasis borono-Mannich (RBR) reaction. The reaction proceeds in very good to excellent yields (84–98%, 17 products) at room temperature with catalyst loadings as low as 1.0 mol%.
2046-2069
79180-79184
Kumar, Prashant
5e332e6f-0450-48c9-9fce-4c663452b8d8
Griffiths, Kieran
91984c79-162c-4653-8521-60b3e76764f2
Lymperopoulou, Smaragda
8a5b1800-8ead-44f6-91ce-5ec6e0f12abd
Kostakis, George E.
dd72c724-c82e-4891-aa68-ccdb42cc6cb8
Kumar, Prashant
5e332e6f-0450-48c9-9fce-4c663452b8d8
Griffiths, Kieran
91984c79-162c-4653-8521-60b3e76764f2
Lymperopoulou, Smaragda
8a5b1800-8ead-44f6-91ce-5ec6e0f12abd
Kostakis, George E.
dd72c724-c82e-4891-aa68-ccdb42cc6cb8

Kumar, Prashant, Griffiths, Kieran, Lymperopoulou, Smaragda and Kostakis, George E. (2016) Tetranuclear Zn2Ln2 coordination clusters as catalysts in the Petasis borono-Mannich multicomponent reaction. RSC Advances, 6 (82), 79180-79184. (doi:10.1039/C6RA17209A).

Record type: Article

Abstract

We report herein for the first time the efficiency of heteronuclear Zn/Ln coordination clusters (CCs) as catalysts for the multicomponent Mannich-type condensation that involves amines, aldehydes and boronic acids, known as the Petasis borono-Mannich (RBR) reaction. The reaction proceeds in very good to excellent yields (84–98%, 17 products) at room temperature with catalyst loadings as low as 1.0 mol%.

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More information

Accepted/In Press date: 10 August 2016
e-pub ahead of print date: 15 August 2016
Organisations: Organic Chemistry: SCF

Identifiers

Local EPrints ID: 403245
URI: http://eprints.soton.ac.uk/id/eprint/403245
ISSN: 2046-2069
PURE UUID: d349fb31-3ea9-4cff-a50f-7112f2c8814d
ORCID for Smaragda Lymperopoulou: ORCID iD orcid.org/0000-0001-7871-4159

Catalogue record

Date deposited: 29 Nov 2016 10:20
Last modified: 15 Mar 2024 03:37

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Contributors

Author: Prashant Kumar
Author: Kieran Griffiths
Author: Smaragda Lymperopoulou ORCID iD
Author: George E. Kostakis

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