²²⁶ Ra determination via the rate of ²²² Rn ingrowth with the Radium Delayed Coincidence Counter (RaDeCC)

Geibert, Walter, Rodellas, Valentí, Annett, Amber, van Beek, Pieter, Garcia-Orellana, Jordi, Hsieh, Yu-Te and Masque, Pere (2013) ²²⁶ Ra determination via the rate of ²²² Rn ingrowth with the Radium Delayed Coincidence Counter (RaDeCC). Limnology and Oceanography: Methods, 11 (11), 594-603. (doi:10.4319/lom.2013.11.594).

Abstract

We present a new method to determine 226 Ra in aqueous environmental samples, based on the rate of ingrowth of 222 Rn from 226 Ra, using the radium delayed coincidence counter (RaDeCC). We use the same instru- ment setup that is used for the determination of 223 Ra and 224 Ra. In contrast to methods published earlier, the approach does not require a modification of the counting equipment, counting separately for 226 Ra, or waiting for radioactive equilibrium. We show that the calibration works from as low as 10 dpm (0.166 Bq) per sample, up to more than 1000 dpm (16.7 Bq). Although uncertainties are larger (typically around 10%) than reported uncertainties for γ counting, liquid scintillation, or mass spectrometry at comparable activities, the simple setup, low cost, and robustness of the method make it a useful approach for underway measurements, combi- nations with short-lived radium isotopes, or monitoring purposes when limited funding or infrastructure is available.

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Contributors

Author: Amber Annett

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