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New developments in the enantioselective synthesis of spiro compounds

New developments in the enantioselective synthesis of spiro compounds
New developments in the enantioselective synthesis of spiro compounds
The enantioselective synthesis of spirocycles has long been pursued by organic chemists. Despite their unique 3D properties and presence in several natural products, the difficulty in their enantioselective synthesis makes them underrepresented in pharmaceutical libraries. Since the first pioneering reports of the enantioselective construction of spirosilanes by Tamao et al., significant effort has been devoted towards the development of new promising asymmetric methodologies. Remarkably, with the advent of organocatalysis, particularly over six years, the reported methodologies for the synthesis of spirocycles have increased exponentially. The aim of this review is to summarize the latest trends and developments in the enantioselective synthesis of spirocompounds during these last six years.
0306-0012
5946-5996
Meazza, Marta
c4665645-8c77-4cfd-aa02-6bcc3341c1aa
Ding, Aishun
be81855a-9636-47f4-8f6d-bd2564bdb2d7
Guo, Hao
2e060524-1e5c-47e7-8ee6-b81d25f82d0d
Yang, Jung Woon
70327194-b21c-402c-83c0-4474fb47db63
Rios, Ramon
609bedf2-e886-4d62-a676-a32b6f8c1441
Meazza, Marta
c4665645-8c77-4cfd-aa02-6bcc3341c1aa
Ding, Aishun
be81855a-9636-47f4-8f6d-bd2564bdb2d7
Guo, Hao
2e060524-1e5c-47e7-8ee6-b81d25f82d0d
Yang, Jung Woon
70327194-b21c-402c-83c0-4474fb47db63
Rios, Ramon
609bedf2-e886-4d62-a676-a32b6f8c1441

Meazza, Marta, Ding, Aishun, Guo, Hao, Yang, Jung Woon and Rios, Ramon (2018) New developments in the enantioselective synthesis of spiro compounds. Chemical Society Reviews, 47 (15), 5946-5996. (doi:10.1039/c6cs00825a).

Record type: Review

Abstract

The enantioselective synthesis of spirocycles has long been pursued by organic chemists. Despite their unique 3D properties and presence in several natural products, the difficulty in their enantioselective synthesis makes them underrepresented in pharmaceutical libraries. Since the first pioneering reports of the enantioselective construction of spirosilanes by Tamao et al., significant effort has been devoted towards the development of new promising asymmetric methodologies. Remarkably, with the advent of organocatalysis, particularly over six years, the reported methodologies for the synthesis of spirocycles have increased exponentially. The aim of this review is to summarize the latest trends and developments in the enantioselective synthesis of spirocompounds during these last six years.

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Revision_2018.05.25_YJW_ - Accepted Manuscript
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Accepted/In Press date: 17 December 2017
e-pub ahead of print date: 29 June 2018

Identifiers

Local EPrints ID: 422303
URI: http://eprints.soton.ac.uk/id/eprint/422303
ISSN: 0306-0012
PURE UUID: 2e33ddcd-08fb-4acf-8408-62e8f15aff23
ORCID for Marta Meazza: ORCID iD orcid.org/0000-0003-4382-0626
ORCID for Ramon Rios: ORCID iD orcid.org/0000-0002-3843-8521

Catalogue record

Date deposited: 20 Jul 2018 16:30
Last modified: 16 Mar 2024 06:50

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Contributors

Author: Marta Meazza ORCID iD
Author: Aishun Ding
Author: Hao Guo
Author: Jung Woon Yang
Author: Ramon Rios ORCID iD

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