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Electrical switching of magnetic polarity in a multiferroic BiFeO3 device at room temperature

Electrical switching of magnetic polarity in a multiferroic BiFeO3 device at room temperature
Electrical switching of magnetic polarity in a multiferroic BiFeO3 device at room temperature
We have directly imaged reversible electrical switching of the cycloidal rotation direction (magnetic polarity) in a (111)pc−BiFeO3 epitaxial-film device at room temperature by nonresonant x-ray magnetic scattering. Consistent with previous reports, fully relaxed (111)pc−BiFeO3 epitaxial films consisting of a single ferroelectric domain are found to comprise a submicron-scale mosaic of magnetoelastic domains, all sharing a common direction of the magnetic polarity, which is found to switch reversibly upon reversal of the ferroelectric polarization without any measurable change of the magnetoelastic domain population. A real-space polarimetry map of our device clearly distinguishes between regions of the sample electrically addressed into the two magnetic states with a resolution of a few tens of micron. Contrary to the general belief that the magneto-electric coupling in BiFeO3 is weak, we find that electrical switching has a dramatic effect on the magnetic structure, with the magnetic moments rotating on average by 90° at every cycle.
2331-7019
Waterfield Price, Noah
3274c895-06a8-466a-92f4-2b3c23ff2510
Johnson, Roger D.
5ed9812f-c020-40a3-b1f1-e7a5780ca2d4
Saenrang, Wittawatt
a7576fe7-b839-4531-92bb-d794042acc71
Bombardi, Alexendro
ebbc9264-3bf7-484f-b49d-c8c817a0f0af
Chmiel, Francis P.
2de259aa-a5eb-460c-bfbf-8b44ed02e2bd
Eom, Chang-Beom
6b5660af-2a05-4f7b-bf59-c0385eae72d2
Radaelli, Paolo G.
210d4ab2-ae25-4d5d-bc1e-5fc881dc6006
Waterfield Price, Noah
3274c895-06a8-466a-92f4-2b3c23ff2510
Johnson, Roger D.
5ed9812f-c020-40a3-b1f1-e7a5780ca2d4
Saenrang, Wittawatt
a7576fe7-b839-4531-92bb-d794042acc71
Bombardi, Alexendro
ebbc9264-3bf7-484f-b49d-c8c817a0f0af
Chmiel, Francis P.
2de259aa-a5eb-460c-bfbf-8b44ed02e2bd
Eom, Chang-Beom
6b5660af-2a05-4f7b-bf59-c0385eae72d2
Radaelli, Paolo G.
210d4ab2-ae25-4d5d-bc1e-5fc881dc6006

Waterfield Price, Noah, Johnson, Roger D., Saenrang, Wittawatt, Bombardi, Alexendro, Chmiel, Francis P., Eom, Chang-Beom and Radaelli, Paolo G. (2017) Electrical switching of magnetic polarity in a multiferroic BiFeO3 device at room temperature. Physical Review Applied, 8 (1), [014033]. (doi:10.1103/PhysRevApplied.8.014033).

Record type: Article

Abstract

We have directly imaged reversible electrical switching of the cycloidal rotation direction (magnetic polarity) in a (111)pc−BiFeO3 epitaxial-film device at room temperature by nonresonant x-ray magnetic scattering. Consistent with previous reports, fully relaxed (111)pc−BiFeO3 epitaxial films consisting of a single ferroelectric domain are found to comprise a submicron-scale mosaic of magnetoelastic domains, all sharing a common direction of the magnetic polarity, which is found to switch reversibly upon reversal of the ferroelectric polarization without any measurable change of the magnetoelastic domain population. A real-space polarimetry map of our device clearly distinguishes between regions of the sample electrically addressed into the two magnetic states with a resolution of a few tens of micron. Contrary to the general belief that the magneto-electric coupling in BiFeO3 is weak, we find that electrical switching has a dramatic effect on the magnetic structure, with the magnetic moments rotating on average by 90° at every cycle.

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More information

e-pub ahead of print date: 27 July 2017
Published date: July 2017

Identifiers

Local EPrints ID: 431621
URI: http://eprints.soton.ac.uk/id/eprint/431621
ISSN: 2331-7019
PURE UUID: 7e975460-c096-442e-a6e0-d409a66942ba

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Date deposited: 11 Jun 2019 16:30
Last modified: 16 Mar 2024 02:12

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Contributors

Author: Noah Waterfield Price
Author: Roger D. Johnson
Author: Wittawatt Saenrang
Author: Alexendro Bombardi
Author: Francis P. Chmiel
Author: Chang-Beom Eom
Author: Paolo G. Radaelli

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