Down the microporous rabbit hole of silicoaluminophosphates, recent developments on synthesis, characterization and catalytic applications
Down the microporous rabbit hole of silicoaluminophosphates, recent developments on synthesis, characterization and catalytic applications
Since their invention silicoaluminophosphates (SAPOs) have become by far the most researched class of aluminophosphates due to their commercial use as solid acid catalysts. Currently over 25 different SAPO frameworks have been synthesized, providing a diverse range of confined nanoporous topologies, with distinct acid sites. When combined with emerging synthetic techniques to further modulate these species, there are endless possibilities to tailor SAPO materials for specific catalytic applications. Herein, this Review focuses on developments, and possibilities, from the past decade in the field of SAPO research, with particular attention paid to synthesis, characterization, theoretical studies, and case studies of their catalytic applications. I aim to simultaneously educate and inspire readers at all stages of their career and hope that this Review helps further interest and research into the exciting field of SAPOs.
Electromagnetic radiation, Silicon, chemical synthesis, crystallization, physical and chemical processes
9758-9789
Potter, Matthew
34dee7dc-2f62-4022-bb65-fc7b7fb526d2
4 September 2020
Potter, Matthew
34dee7dc-2f62-4022-bb65-fc7b7fb526d2
Potter, Matthew
(2020)
Down the microporous rabbit hole of silicoaluminophosphates, recent developments on synthesis, characterization and catalytic applications.
ACS Catalysis, 10 (17), .
(doi:10.1021/acscatal.0c02278).
Abstract
Since their invention silicoaluminophosphates (SAPOs) have become by far the most researched class of aluminophosphates due to their commercial use as solid acid catalysts. Currently over 25 different SAPO frameworks have been synthesized, providing a diverse range of confined nanoporous topologies, with distinct acid sites. When combined with emerging synthetic techniques to further modulate these species, there are endless possibilities to tailor SAPO materials for specific catalytic applications. Herein, this Review focuses on developments, and possibilities, from the past decade in the field of SAPO research, with particular attention paid to synthesis, characterization, theoretical studies, and case studies of their catalytic applications. I aim to simultaneously educate and inspire readers at all stages of their career and hope that this Review helps further interest and research into the exciting field of SAPOs.
Text
MEP ACS Catalysis SAPO Review
- Accepted Manuscript
More information
e-pub ahead of print date: 19 July 2020
Published date: 4 September 2020
Additional Information:
Funding Information:
The author has given approval to the final version of the manuscript. M.E.P. is currently funded by Total on the “Consortium on Metal Nanocatalysis” project.
Publisher Copyright:
Copyright © 2020 American Chemical Society.
Keywords:
Electromagnetic radiation, Silicon, chemical synthesis, crystallization, physical and chemical processes
Identifiers
Local EPrints ID: 443634
URI: http://eprints.soton.ac.uk/id/eprint/443634
ISSN: 2155-5435
PURE UUID: 0d06f53d-fcd5-43f3-96b4-09679c8c5285
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Date deposited: 07 Sep 2020 16:30
Last modified: 17 Mar 2024 05:51
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