Nano-second exciton-polariton lasing in organic microcavities
Nano-second exciton-polariton lasing in organic microcavities
Organic semiconductors are a promising platform for ambient polaritonics. Several applications, such as polariton routers, and many-body condensed matter phenomena are currently hindered due to the ultra-short polariton lifetimes in organics. Here, we employ a single-shot dispersion imaging technique, using 4 ns long non-resonant excitation pulses, to study polariton lasing in a λ/2 planar organic microcavity filled with BODIPY-Br dye molecules. At a power threshold density of 1.5 MW/cm 2, we observe the transition to a quasi-steady state, 1.2 ns long-lived, single-mode polariton lasing and the concomitant superlinear increase in photoluminescence, spectral line-narrowing, and energy blueshift.
Putintsev, Anton
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Zasedatelev, Anton
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McGhee, Kirsty E.
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Cookson, Tamsin
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Georgiou, Kyriacos
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Sannikov, Denis A.
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Lidzey, David G
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Lagoudakis, Pavlos
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Putintsev, Anton
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Zasedatelev, Anton
b8f8265a-58a1-48c8-abf5-68e4e6ef8f70
McGhee, Kirsty E.
28b64dac-b1a1-442d-ac3d-ee2fe41e005f
Cookson, Tamsin
70c15876-7c6d-4de5-a0ce-cc4beb12a324
Georgiou, Kyriacos
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Sannikov, Denis A.
8712f2bf-5b5b-4017-8eee-a8a20001c1a9
Lidzey, David G
073d4479-103d-401c-bcb2-293decbb9114
Lagoudakis, Pavlos
ea50c228-f006-4edf-8459-60015d961bbf
Putintsev, Anton, Zasedatelev, Anton, McGhee, Kirsty E., Cookson, Tamsin, Georgiou, Kyriacos, Sannikov, Denis A., Lidzey, David G and Lagoudakis, Pavlos
(2020)
Nano-second exciton-polariton lasing in organic microcavities.
Applied Physics Letters, 117 (12), [123302].
(doi:10.1063/5.0019195).
Abstract
Organic semiconductors are a promising platform for ambient polaritonics. Several applications, such as polariton routers, and many-body condensed matter phenomena are currently hindered due to the ultra-short polariton lifetimes in organics. Here, we employ a single-shot dispersion imaging technique, using 4 ns long non-resonant excitation pulses, to study polariton lasing in a λ/2 planar organic microcavity filled with BODIPY-Br dye molecules. At a power threshold density of 1.5 MW/cm 2, we observe the transition to a quasi-steady state, 1.2 ns long-lived, single-mode polariton lasing and the concomitant superlinear increase in photoluminescence, spectral line-narrowing, and energy blueshift.
Text
Nano-second exciton-polariton lasing in organic microcavities
- Accepted Manuscript
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Accepted/In Press date: 3 September 2020
e-pub ahead of print date: 21 September 2020
Additional Information:
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Local EPrints ID: 444638
URI: http://eprints.soton.ac.uk/id/eprint/444638
ISSN: 0003-6951
PURE UUID: 3bcd62ac-d0fb-4dee-a530-55192e8e0208
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Date deposited: 28 Oct 2020 17:30
Last modified: 10 Jan 2022 03:18
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Contributors
Author:
Anton Putintsev
Author:
Kirsty E. McGhee
Author:
Tamsin Cookson
Author:
Kyriacos Georgiou
Author:
Denis A. Sannikov
Author:
David G Lidzey
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