READ ME File For 'Widely-tunable synchronisation-free picosecondlaser source for multimodal CARS, SHG andtwo-photon microscopy' Dataset DOI: https://doi.org/10.5258/SOTON/D1662 ReadMe Author: Duanyang Xu, University of Southampton [ORCID ID orcid.org/0000-0002-9122-1049] This dataset supports the publication: AUTHORS: Duanyang Xu, Sijing Liang, Lin Xu, Konstantinos Bourdakos, Peter Johnson, James Read, Jonathan Price, Sumeet Mahajan, and David Richardson TITLE: Widely-tunable synchronisation-free picosecond laser source for multimodal CARS, SHG and two-photon microscopy JOURNAL Biomedical Optics Express PAPER DOI https://doi.org/10.1364/BOE.411620 This dataset contains experimental data for the paper. The figures are as follows: Fig. 2 a) Auto-correlation measurement of EE source (Emerald Engine pump laser)(1031 nm) (green) and OPA-SHG output (red). AC, auto-correlation. (b) Spectrum ofthe Stokes beam (OPA pump source) and TLS output (OPA seed). Fig. 3 OPA output (solid square), SHG output (solid circle) and OPA gain (emptysquare, blue) as a function of pump power (a) or seed power (b). Spectra and power of CW seeded OPA (a) and SHG (b) later used as the tunable CARS Pump beam. Fig. 4 a) Measured CARS spectra of polystyrene beads overlayed with the spontaneous Raman spectra. Date of data collection: 06/2019-03/2020 Information about geographic location of data collection: University of Southampton, U.K. Licence: CC BY Related projects: Engineering and Physical Sciences Research Council (EPSRCUK) through the Airguide Photonics Program Grant (EP/P030181/1), by grants EP/R041814/1,EP/P027644/1, EP/P012248/1, EP/T020997/1 and by the US Air Force Office of Scientific Research (AFOSR) project FA9550-14-1-0382, ERC grant NanoChemBioVision (638258). Date that the file was created: December 2020