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Identification of the surface species responsible for N2O formation from the chemisorption of NO on Rh/alumina

Identification of the surface species responsible for N2O formation from the chemisorption of NO on Rh/alumina
Identification of the surface species responsible for N2O formation from the chemisorption of NO on Rh/alumina
Energy dispersive EXAFS (EDE) and diffuse reflectance infrared spectroscopy (DRIFTS) are combined synchronously at high time resolution (17 Hz) to probe how NO(g) reacts with gamma-Al2O3 supported, metallic Rh nanoparticles of an average 11 A diameter; a bent nitrosyl species is considered to be the key to the formation of N2O.
energy loss characterization, rh catalysts, heterogeneous catalysts, rh/al2o3 catalysts, exhaust catalysis, dispersive exafs, ft-ir, co, rh(111), interconversion
1463-9076
246-249
Newton, Mark A.
73aab2af-4641-47f3-89ad-3b7d3026164f
Dent, Andrew J.
24c2a218-cb0e-4193-af0b-3ff1dc42b552
Fiddy, Steven G.
f6c255cf-6aa1-4798-85ca-1a2ccdaa1186
Jyoti, Bhrat
9e00e347-0864-48fa-9bb8-f44f98161fd0
Evans, John
43f91d41-73e9-4611-b7a8-f649d7ae9e2b
Newton, Mark A.
73aab2af-4641-47f3-89ad-3b7d3026164f
Dent, Andrew J.
24c2a218-cb0e-4193-af0b-3ff1dc42b552
Fiddy, Steven G.
f6c255cf-6aa1-4798-85ca-1a2ccdaa1186
Jyoti, Bhrat
9e00e347-0864-48fa-9bb8-f44f98161fd0
Evans, John
43f91d41-73e9-4611-b7a8-f649d7ae9e2b

Newton, Mark A., Dent, Andrew J., Fiddy, Steven G., Jyoti, Bhrat and Evans, John (2007) Identification of the surface species responsible for N2O formation from the chemisorption of NO on Rh/alumina. Physical Chemistry Chemical Physics, 9 (2), 246-249. (doi:10.1039/b613251k).

Record type: Article

Abstract

Energy dispersive EXAFS (EDE) and diffuse reflectance infrared spectroscopy (DRIFTS) are combined synchronously at high time resolution (17 Hz) to probe how NO(g) reacts with gamma-Al2O3 supported, metallic Rh nanoparticles of an average 11 A diameter; a bent nitrosyl species is considered to be the key to the formation of N2O.

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More information

Published date: 2007
Keywords: energy loss characterization, rh catalysts, heterogeneous catalysts, rh/al2o3 catalysts, exhaust catalysis, dispersive exafs, ft-ir, co, rh(111), interconversion

Identifiers

Local EPrints ID: 44593
URI: http://eprints.soton.ac.uk/id/eprint/44593
ISSN: 1463-9076
PURE UUID: e85861f9-2883-4567-ae42-be2f4bfad714

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Date deposited: 02 Mar 2007
Last modified: 15 Mar 2024 09:05

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Contributors

Author: Mark A. Newton
Author: Andrew J. Dent
Author: Steven G. Fiddy
Author: Bhrat Jyoti
Author: John Evans

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