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Strong coupling between localized plasmons and organic excitons in metal nanovoids

Strong coupling between localized plasmons and organic excitons in metal nanovoids
Strong coupling between localized plasmons and organic excitons in metal nanovoids
Hybrid emitting exciton-plasmonic composites are constructed by coating arrays of spherical nanovoids embedded in a gold film with organic semiconducting molecular J-aggregate films. In such plasmonic crystals, localized plasmons confined inside the voids can be excited. We report the first observation of polaritonic spectral narrowing and strong coupling between localized plasmons and J-aggregate excitons with Rabi splittings of 230 meV at room temperature.
enhanced raman-scattering, fluorescence, microcavity, emission, films, light, dyes
0031-9007
266808-[4pp]
Sugawara, Y.
585b662a-5e52-4e03-ba20-8a9f602fcb4b
Kelf, T.A.
f28ac06f-3dda-4ad7-ac70-470111d46f64
Baumberg, J.J.
78e1ea7e-8c70-404c-bf84-59aafe75cd07
Abdelsalam, M.E.
94ec836b-cf24-4b21-9a6c-c3436b8ef3b2
Bartlett, P.N.
d99446db-a59d-4f89-96eb-f64b5d8bb075
Sugawara, Y.
585b662a-5e52-4e03-ba20-8a9f602fcb4b
Kelf, T.A.
f28ac06f-3dda-4ad7-ac70-470111d46f64
Baumberg, J.J.
78e1ea7e-8c70-404c-bf84-59aafe75cd07
Abdelsalam, M.E.
94ec836b-cf24-4b21-9a6c-c3436b8ef3b2
Bartlett, P.N.
d99446db-a59d-4f89-96eb-f64b5d8bb075

Sugawara, Y., Kelf, T.A., Baumberg, J.J., Abdelsalam, M.E. and Bartlett, P.N. (2006) Strong coupling between localized plasmons and organic excitons in metal nanovoids. Physical Review Letters, 97 (26), 266808-[4pp]. (doi:10.1103/PhysRevLett.97.266808).

Record type: Article

Abstract

Hybrid emitting exciton-plasmonic composites are constructed by coating arrays of spherical nanovoids embedded in a gold film with organic semiconducting molecular J-aggregate films. In such plasmonic crystals, localized plasmons confined inside the voids can be excited. We report the first observation of polaritonic spectral narrowing and strong coupling between localized plasmons and J-aggregate excitons with Rabi splittings of 230 meV at room temperature.

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Published date: 29 December 2006
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Keywords: enhanced raman-scattering, fluorescence, microcavity, emission, films, light, dyes
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Identifiers

Local EPrints ID: 44598
URI: http://eprints.soton.ac.uk/id/eprint/44598
DOI: doi:10.1103/PhysRevLett.97.266808
ISSN: 0031-9007
PURE UUID: b03ff7cc-ccdd-4633-a537-4ad626f0b8d1
ORCID for P.N. Bartlett: ORCID iD orcid.org/0000-0002-7300-6900

Catalogue record

Date deposited: 05 Mar 2007
Last modified: 16 Mar 2024 02:43

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Contributors

Author: Y. Sugawara
Author: T.A. Kelf
Author: J.J. Baumberg
Author: M.E. Abdelsalam
Author: P.N. Bartlett ORCID iD

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