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AI3SD Video: When charge transport data are a worm – a transfer learning approach for unsupervised data classification

AI3SD Video: When charge transport data are a worm – a transfer learning approach for unsupervised data classification
AI3SD Video: When charge transport data are a worm – a transfer learning approach for unsupervised data classification
Advanced data analysis methodologies, and in particular dimensionality reduction techniques, are now used more and more widely in the single-molecule charge transport community. They allow for comprehensive exploration of large datasets, where data display significant variance and sometimes contain (unknown) sub-populations. To this end, unsupervised approaches, which do not rely on class labels or pre-defined expectations can be advantageous. Multi-Parameter Vector Classification (MPVC) is one example and PCA-based methods have also been employed in this context [1,2,3]. We have recently shown how Transfer Learning may be employed to identify and quantify hidden features in single-molecule charge transport data [3]. Using open-access neural networks such as AlexNet, trained on millions of seemingly unrelated image data, feature recognition then does not require network training with application-specific data. Instead, the network recognises features in the input that it had learned in other contexts and, for example, identifies different shapes in conductance-distance traces as images of different worm species. Thus, our results show how Deep Learning methodologies can readily be employed for unsupervised data classification, even if the amount of problem-specific, ‘own’ data is limited.

[1] M Lemmer, MS Inkpen, K Kornysheva, NJ Long, T Albrecht, “Unsupervised vector-based classification of single-molecule charge transport data”, Nat. Comm. 2016, 7, 12922.
[2] T Albrecht, G Slabaugh, E Alonso, SMMR Al-Arif, “Deep learning for single-molecule science”, Nanotechnology 2017, 28 (42), 423001.
[3] A Vladyka, T Albrecht, “Unsupervised classification of single-molecule data with autoencoders and transfer learning”, Mach. Learn.: Sci. Technol. 2020, 1, 035013.
AI, AI3SD Event, Artificial Intelligence, Chemical Tomography, Chemistry, Machine Intelligence, Machine Learning, ML, Molecules Discovery, Prediction, Scientific Discovery
Albrecht, Tim
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Kanza, Samantha
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Frey, Jeremy G.
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Niranjan, Mahesan
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Hooper, Victoria
af1a99f1-7848-4d5c-a4b5-615888838d84
Albrecht, Tim
94446f17-f189-45d4-852a-a5a5c0a6d2e3
Kanza, Samantha
b73bcf34-3ff8-4691-bd09-aa657dcff420
Frey, Jeremy G.
ba60c559-c4af-44f1-87e6-ce69819bf23f
Niranjan, Mahesan
5cbaeea8-7288-4b55-a89c-c43d212ddd4f
Hooper, Victoria
af1a99f1-7848-4d5c-a4b5-615888838d84

Albrecht, Tim (2020) AI3SD Video: When charge transport data are a worm – a transfer learning approach for unsupervised data classification. Kanza, Samantha, Frey, Jeremy G., Niranjan, Mahesan and Hooper, Victoria (eds.) AI3SD Winter Seminar Series, , Online. 18 Nov 2020 - 21 Apr 2021 . (doi:10.5258/SOTON/P0083).

Record type: Conference or Workshop Item (Other)

Abstract

Advanced data analysis methodologies, and in particular dimensionality reduction techniques, are now used more and more widely in the single-molecule charge transport community. They allow for comprehensive exploration of large datasets, where data display significant variance and sometimes contain (unknown) sub-populations. To this end, unsupervised approaches, which do not rely on class labels or pre-defined expectations can be advantageous. Multi-Parameter Vector Classification (MPVC) is one example and PCA-based methods have also been employed in this context [1,2,3]. We have recently shown how Transfer Learning may be employed to identify and quantify hidden features in single-molecule charge transport data [3]. Using open-access neural networks such as AlexNet, trained on millions of seemingly unrelated image data, feature recognition then does not require network training with application-specific data. Instead, the network recognises features in the input that it had learned in other contexts and, for example, identifies different shapes in conductance-distance traces as images of different worm species. Thus, our results show how Deep Learning methodologies can readily be employed for unsupervised data classification, even if the amount of problem-specific, ‘own’ data is limited.

[1] M Lemmer, MS Inkpen, K Kornysheva, NJ Long, T Albrecht, “Unsupervised vector-based classification of single-molecule charge transport data”, Nat. Comm. 2016, 7, 12922.
[2] T Albrecht, G Slabaugh, E Alonso, SMMR Al-Arif, “Deep learning for single-molecule science”, Nanotechnology 2017, 28 (42), 423001.
[3] A Vladyka, T Albrecht, “Unsupervised classification of single-molecule data with autoencoders and transfer learning”, Mach. Learn.: Sci. Technol. 2020, 1, 035013.

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More information

Published date: 16 December 2020
Additional Information: Tim studied Chemistry at the University of Essen in Germany from 1995-2000. Following brief research visits at the European Joint Research Centre in Ispra in Italy and the University of California at Berkeley, Tim graduated with a Diploma in Chemistry (equivalent to a Masters degree) in early 2000. After graduating, Tim joined Peter Hildebrandt’s group at the Max-Planck Institute for Radiation Chemistry (now Bioinorganic Chemistry) in 2000. Tim worked on charge transfer processes in natural and artificial heme proteins on metal surfaces using SER(R)S, single-crystal electrochemistry and electrochemical STM (in Jens Ulstrup’s group at the Technical Institute of Denmark (DTU). He obtained his PhD from the Technical University (TU) of Berlin in 2003 and afterwards returned to Ulstrup’s group as a postdoctoral fellow. In 2006, he moved to London to take up a lecturer position in Interfacial and Analytical Sciences in the Chemistry Department at Imperial College, where he was made Senior Lecturer in 2011 and then Reader in 2014. In 2017, Tim joined the faculty in the School of Chemistry at Birmingham University as Chair of Physical Chemistry and has been the School of Chemistry’s Director of Research since 2018. He is the coordinator of the School’s Interest Group “Data and Machine Intelligence”.
Venue - Dates: AI3SD Winter Seminar Series, , Online, 2020-11-18 - 2021-04-21
Keywords: AI, AI3SD Event, Artificial Intelligence, Chemical Tomography, Chemistry, Machine Intelligence, Machine Learning, ML, Molecules Discovery, Prediction, Scientific Discovery

Identifiers

Local EPrints ID: 448779
URI: http://eprints.soton.ac.uk/id/eprint/448779
PURE UUID: 85b2279a-8080-417b-b344-3c3c6b8d0bd0
ORCID for Samantha Kanza: ORCID iD orcid.org/0000-0002-4831-9489
ORCID for Jeremy G. Frey: ORCID iD orcid.org/0000-0003-0842-4302
ORCID for Mahesan Niranjan: ORCID iD orcid.org/0000-0001-7021-140X

Catalogue record

Date deposited: 05 May 2021 16:44
Last modified: 17 Mar 2024 03:51

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Contributors

Author: Tim Albrecht
Editor: Samantha Kanza ORCID iD
Editor: Jeremy G. Frey ORCID iD
Editor: Mahesan Niranjan ORCID iD
Editor: Victoria Hooper

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