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Accounting for surface waves improves gas flux estimation at high wind speed in a large lake

Accounting for surface waves improves gas flux estimation at high wind speed in a large lake
Accounting for surface waves improves gas flux estimation at high wind speed in a large lake
The gas transfer velocity (k) is a major source of uncertainty when assessing the magnitude of lake gas exchange with the atmosphere. For the diversity of existing empirical and process-based k models, the transfer velocity increases with the level of turbulence near the air-water interface. However, predictions for k can vary by a factor of 2 among different models. Near-surface turbulence results from the action of wind shear, surface waves and buoyancy-driven convection. Wind shear has long been identified as a key driver, while recent lake studies have shifted the focus towards the role of convection, particularly in small lakes. In large lakes, wind fetch can however be long enough to generate surface waves and contribute to enhance gas transfer, as widely recognised in oceanographic studies. Here, field values for gas transfer velocity were computed in a large hardwater lake, Lake Geneva, from CO2 fluxes measured with an automated (forced diffusion) flux chamber and CO2 partial pressure measured with high frequency sensors. k estimates were compared to a set of reference limnological and oceanic k models. Our analysis reveals that accounting for surface waves generated during windy events significantly improves the accuracy of k estimates in this large lake. The improved k model is then used to compute k over a one-year time-period. Results show that episodic extreme events with surface waves (6 % occurrence, significant wave height > 0.4 m) can generate more than 20 % of annual cumulative k and more than 25 % of annual net CO2 fluxes in Lake Geneva. We conclude that for lakes whose fetch can exceed 15 km, k-models need to integrate the effect of surface waves.
2190-4979
1169–1189
Perolo, Pascal
1c35f952-142e-4f36-add3-c6f1e6a5b18c
Castro, Bieito Fernández
8017e93c-d5ee-4bba-b443-9c72ca512d61
Escoffier, Nicolas
39bdfefa-28bb-4d1a-b66c-ff478e88ded3
Lambert, Thibault
f99bd1ec-f94a-489e-bb49-ad575d10157b
Bouffard, Damien
a3eb0e77-974e-40b5-a122-388e1c15704b
Perga, Marie-Elodie
a04e0382-5b17-4730-8b88-47c3d902cd61
Perolo, Pascal
1c35f952-142e-4f36-add3-c6f1e6a5b18c
Castro, Bieito Fernández
8017e93c-d5ee-4bba-b443-9c72ca512d61
Escoffier, Nicolas
39bdfefa-28bb-4d1a-b66c-ff478e88ded3
Lambert, Thibault
f99bd1ec-f94a-489e-bb49-ad575d10157b
Bouffard, Damien
a3eb0e77-974e-40b5-a122-388e1c15704b
Perga, Marie-Elodie
a04e0382-5b17-4730-8b88-47c3d902cd61

Perolo, Pascal, Castro, Bieito Fernández, Escoffier, Nicolas, Lambert, Thibault, Bouffard, Damien and Perga, Marie-Elodie (2021) Accounting for surface waves improves gas flux estimation at high wind speed in a large lake. Earth System Dynamics, 12 (4), 1169–1189. (doi:10.5194/esd-2021-30).

Record type: Article

Abstract

The gas transfer velocity (k) is a major source of uncertainty when assessing the magnitude of lake gas exchange with the atmosphere. For the diversity of existing empirical and process-based k models, the transfer velocity increases with the level of turbulence near the air-water interface. However, predictions for k can vary by a factor of 2 among different models. Near-surface turbulence results from the action of wind shear, surface waves and buoyancy-driven convection. Wind shear has long been identified as a key driver, while recent lake studies have shifted the focus towards the role of convection, particularly in small lakes. In large lakes, wind fetch can however be long enough to generate surface waves and contribute to enhance gas transfer, as widely recognised in oceanographic studies. Here, field values for gas transfer velocity were computed in a large hardwater lake, Lake Geneva, from CO2 fluxes measured with an automated (forced diffusion) flux chamber and CO2 partial pressure measured with high frequency sensors. k estimates were compared to a set of reference limnological and oceanic k models. Our analysis reveals that accounting for surface waves generated during windy events significantly improves the accuracy of k estimates in this large lake. The improved k model is then used to compute k over a one-year time-period. Results show that episodic extreme events with surface waves (6 % occurrence, significant wave height > 0.4 m) can generate more than 20 % of annual cumulative k and more than 25 % of annual net CO2 fluxes in Lake Geneva. We conclude that for lakes whose fetch can exceed 15 km, k-models need to integrate the effect of surface waves.

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Submitted date: 7 May 2021
e-pub ahead of print date: 17 November 2021
Published date: 17 November 2021

Identifiers

Local EPrints ID: 449805
URI: http://eprints.soton.ac.uk/id/eprint/449805
ISSN: 2190-4979
PURE UUID: 39eb8a10-3cad-4f38-9dbf-f6a8ba54b880
ORCID for Bieito Fernández Castro: ORCID iD orcid.org/0000-0001-7797-854X

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Date deposited: 17 Jun 2021 16:36
Last modified: 17 Mar 2024 04:04

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Contributors

Author: Pascal Perolo
Author: Nicolas Escoffier
Author: Thibault Lambert
Author: Damien Bouffard
Author: Marie-Elodie Perga

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