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Roadmap on inorganic perovskites for energy applications

Roadmap on inorganic perovskites for energy applications
Roadmap on inorganic perovskites for energy applications
Inorganic perovskites exhibit many important physical properties such as ferroelectricity, magnetoresistance and superconductivity as well their importance as energy materials. Many of the most important energy materials are inorganic perovskites and find application in batteries, fuel cells, photocatalysts, catalysis, thermoelectrics and solar thermal. In all these applications, perovskite oxides, or their derivatives offer highly competitive performance, often state of the art and so tend to dominate research into energy material. In the following sections, we review these functionalities in turn seeking to facilitate the interchange of ideas between domains. The potential for improvement is explored and we highlight the importance of both detailed modelling and in situ and operando studies in taking these materials forward.
Fuel cells, catalysis, energy, perovskites, solar fuels, thermoelectrics, water splitting
2515-7655
Irvine, John
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Rupp, Jennifer L.M.
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Li, Gang
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Xu, Xiaoxiang
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Haile, Sossina
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Qian, Xin
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Snyder, Alem
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Freer, Robert
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Ekren, Dursun
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Skinner, Stephen
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Celikbilek, Ozden
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Chen, Shigang
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Tao, Shanwen
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Shin, Tae Ho
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O’Hayre, Ryan
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Huang, Jake
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Duan, Chuancheng
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Papac, Meagan
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Li, Shuangbin
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Celorrio, Verónica
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Russell, Andrea E.
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Hayden, Brian
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Nolan, Hugo
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Huang, Xiubing
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Wang, Ge
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Metcalfe, Ian
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Neagu, Dragos
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Garcia Martín, Susana
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Irvine, John
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Rupp, Jennifer L.M.
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Li, Gang
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Xu, Xiaoxiang
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Haile, Sossina
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Qian, Xin
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Snyder, Alem
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Freer, Robert
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Ekren, Dursun
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Skinner, Stephen
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Celikbilek, Ozden
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Chen, Shigang
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Tao, Shanwen
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Shin, Tae Ho
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O’Hayre, Ryan
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Huang, Jake
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Duan, Chuancheng
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Papac, Meagan
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Li, Shuangbin
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Celorrio, Verónica
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Russell, Andrea E.
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Hayden, Brian
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Nolan, Hugo
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Huang, Xiubing
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Wang, Ge
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Metcalfe, Ian
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Neagu, Dragos
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Garcia Martín, Susana
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Irvine, John, Rupp, Jennifer L.M., Li, Gang, Xu, Xiaoxiang, Haile, Sossina, Qian, Xin, Snyder, Alem, Freer, Robert, Ekren, Dursun, Skinner, Stephen, Celikbilek, Ozden, Chen, Shigang, Tao, Shanwen, Shin, Tae Ho, O’Hayre, Ryan, Huang, Jake, Duan, Chuancheng, Papac, Meagan, Li, Shuangbin, Celorrio, Verónica, Russell, Andrea E., Hayden, Brian, Nolan, Hugo, Huang, Xiubing, Wang, Ge, Metcalfe, Ian, Neagu, Dragos and Garcia Martín, Susana (2021) Roadmap on inorganic perovskites for energy applications. Journal of Physics: Energy, 3 (3), [031502]. (doi:10.1088/2515-7655/abff18).

Record type: Article

Abstract

Inorganic perovskites exhibit many important physical properties such as ferroelectricity, magnetoresistance and superconductivity as well their importance as energy materials. Many of the most important energy materials are inorganic perovskites and find application in batteries, fuel cells, photocatalysts, catalysis, thermoelectrics and solar thermal. In all these applications, perovskite oxides, or their derivatives offer highly competitive performance, often state of the art and so tend to dominate research into energy material. In the following sections, we review these functionalities in turn seeking to facilitate the interchange of ideas between domains. The potential for improvement is explored and we highlight the importance of both detailed modelling and in situ and operando studies in taking these materials forward.

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Accepted/In Press date: 7 May 2021
Published date: 22 July 2021
Additional Information: Funding Information: The authors are grateful to the EPSRC for the provision of funding for this work (EP/H043462, EP/I036230/1, EP/L014068/1, EP/L017695/1 acknowledged by R F). All research data supporting this publication are directly available within the publication. Funding Information: The authors thank National Natural Science Foundation of China (Nos. 51825204,51629201, 51972233), the Key Research Program of Frontier Sciences CAS (QYZDB-SSW-JSC039), Natural Science Foundation of Shanghai (Grant No. 19ZR1459200), Shanghai Science and Technology Commission (14DZ2261100) and the Fundamental Research Funds for the Central Universities for the financial support. Funding Information: This work was supported by funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie Grant Agreement No. 836503. Funding Information: R O, J H and C D acknowledge funding from the Advanced Research Projects Agency–Energy (ARPA-E) through the REFUEL (Award DE-AR0000808) and REBELS programs (Award DE-AR0000493). R O and M P acknowledge funding from the Army Research Office under Grant Number W911NF-17-1-0051. Funding Information: The authors thank E Mastronardo for providing raw data published in [16], and C Wolverton for valuable discussions of ab initio computational approaches. Financial support has been provided by the US Department of Energy, Office of Energy Efficiency and Renewable Energy under DE-EE0008089. Funding Information: I thank the Agencia Estatal de Investigación (AEI)/Fondo Europeo de Desarrollo Regional (FEDER/UE) for funding the Project PID2019-106662RB-C44 and the European Union for the Marie Curie fellowship (Human Capital and Mobility Program) that allowed me to start working in Li-perovskites at the University of Aberdeen (Department of Chemistry) back in 1993. Funding Information: The authors thank EPSRC (Grant No. EP/G030995/1) for funding. Funding Information: The authors are grateful for the financial supports from the National Natural Science Foundation of China (51802015), 111 Project (B170003) and the Fundamental Research Funds for the Central Universities (FRF-TP-20-005A3). Funding Information: This work was supported by the Technology Innovation Program (Grant No. 20004963) the Korea Evaluation Institute of Industrial Technology (KEIT) and the Ministry or Trade, industry & Energy (MOTIE) of the Republic of Korea. We thank EPSRC (EP/P007821/1). Publisher Copyright: © 2021 IOP Publishing Ltd
Keywords: Fuel cells, catalysis, energy, perovskites, solar fuels, thermoelectrics, water splitting

Identifiers

Local EPrints ID: 450773
URI: http://eprints.soton.ac.uk/id/eprint/450773
ISSN: 2515-7655
PURE UUID: c857cc2e-8653-4af9-91a9-eb18034326a1
ORCID for Andrea E. Russell: ORCID iD orcid.org/0000-0002-8382-6443
ORCID for Brian Hayden: ORCID iD orcid.org/0000-0002-7762-1812
ORCID for Hugo Nolan: ORCID iD orcid.org/0000-0003-3262-6860

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Date deposited: 11 Aug 2021 16:30
Last modified: 30 Aug 2024 01:35

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Contributors

Author: John Irvine
Author: Jennifer L.M. Rupp
Author: Gang Li
Author: Xiaoxiang Xu
Author: Sossina Haile
Author: Xin Qian
Author: Alem Snyder
Author: Robert Freer
Author: Dursun Ekren
Author: Stephen Skinner
Author: Ozden Celikbilek
Author: Shigang Chen
Author: Shanwen Tao
Author: Tae Ho Shin
Author: Ryan O’Hayre
Author: Jake Huang
Author: Chuancheng Duan
Author: Meagan Papac
Author: Shuangbin Li
Author: Verónica Celorrio
Author: Brian Hayden ORCID iD
Author: Hugo Nolan ORCID iD
Author: Xiubing Huang
Author: Ge Wang
Author: Ian Metcalfe
Author: Dragos Neagu
Author: Susana Garcia Martín

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