The University of Southampton
University of Southampton Institutional Repository

Assuring the integrity of offshore carbon dioxide storage

Assuring the integrity of offshore carbon dioxide storage
Assuring the integrity of offshore carbon dioxide storage
Carbon capture and storage is a key mitigation strategy proposed for keeping the global temperature rise below 1.5 °C. Offshore storage can provide up to 13% of the global CO2 reduction required to achieve the Intergovernmental Panel on Climate Change goals. The public must be assured that potential leakages from storage reservoirs can be detected and that therefore the CO2 is safely contained. We conducted a controlled release of 675 kg CO2 within sediments at 120 m water depth, to simulate a leak and test novel detection, quantification and attribution approaches. We show that even at a very low release rate (6 kg day−1), CO2 can be detected within sediments and in the water column. Alongside detection we show the fluxes of both dissolved and gaseous CO2 can be quantified. The CO2 source was verified using natural and added tracers. The experiment demonstrates that existing technologies and techniques can detect, attribute and quantify any escape of CO2 from sub-seabed reservoirs as required for public assurance, regulatory oversight and emissions trading schemes.
Carbon Capture and Storage, Carbon dioxide, MONITORING, Marine Carbon Capture and Storage, measurement, verification
1364-0321
Connelly, Douglas
a0d5c204-2cda-464a-850d-af1408d9de5f
Bull, Jonathan
974037fd-544b-458f-98cc-ce8eca89e3c8
Flohr, Anita
1e293a22-bdba-408e-9608-fed8b65e4e79
Koopmans, Dirk
abfee455-7f02-4de7-a4db-5b25cd7d8e03
Blackford, Jerry
0bd48334-2280-4209-aa74-8f411149b754
White, Paul
2dd2477b-5aa9-42e2-9d19-0806d994eaba
James, Rachael
79aa1d5c-675d-4ba3-85be-fb20798c02f4
Pearce, Chris
c8a35d08-42ce-46c7-82a6-7aba34890355
lichtschlag, Anna
56dc1ed4-7301-4e3f-9650-7c08162517cd
Achterberg, Eric
da742b45-3cf2-4ab4-8a51-1da00254c686
de Beer, Dirk
060ba2b9-7984-47b3-a206-c43f8b0fd110
Roche, Ben
08938cb1-4901-4f45-ba9a-aba53ed4ef7f
Li, Jianghui
9c589194-00fa-4d42-abaf-53a32789cc5e
Saw, Kevin
d17fe3b0-a61d-4ffc-bcf1-f24abd26e477
Alendal, G
f3063723-5b3d-4a38-adef-77a0663b0afc
Alvesen, H
0d510640-df81-4298-aa1a-4f14727db2df
Brown, R
aa3db44f-5ed8-475f-a28c-988031ff237e
Borisov, Sergei
6d842cf5-db81-440c-a6f4-c6831e020982
Bottner, Christoph
83baec2f-b6a6-4e0d-9e62-5da261de52fc
Cazenave, Pierre
869028e0-0c5d-4dc0-9e99-4d5b0d15747c
Chen, Baixin
001da024-c7b9-4629-a3d7-ccac1809d183
Dale, A
6c26d2d2-ff77-47bc-b962-60a7b861df1a
Dean, Marcella
561ef3e4-7234-4be5-bea8-396becfa247a
Dewar, Marius
5f898f03-2910-40ba-8b82-f6c755580657
Esposito, M
d87109c6-7315-46ac-b219-2a4c56870321
Gros, J
b6d6b05c-d170-46e3-9c39-b47bb1010687
Hanz, R
321f373e-7079-4afa-8954-fbf6ec88cf03
Haeckel, Matthias
dd9d005c-e484-4b57-a992-1d5cb7c3a3a7
Hosking, Brett
1d665df5-7c75-43c1-8b4a-ae4df5b8678c
Huvenne, veerle
2968611c-22f7-40ea-9e30-13ebf214b67b
Karstens, Jens
d87f50cb-dd8b-4b8f-85b0-3ad046642eb3
Le Bas, Tim
af315ced-85e0-4ec8-abfd-d80069685bb6
Leighton, Timothy
3e5262ce-1d7d-42eb-b013-fcc5c286bbae
Linke, Peter
f5865fb6-dbce-4072-8e6f-4fd313d0de71
Loucaides, S
9eeb8c5c-0212-4769-84b9-f860c9b96356
Matter, Juerg
abb60c24-b6cb-4d1a-a108-6fc51ee20395
Monk, S
4f47a781-581e-4dd0-aa58-4ec63e43776c
Mowlem, Matthew
ef893d5a-8244-4ab5-b605-11e0cac45b7a
Oleynik, A
55c41da0-c80c-46bc-916e-950c2cb0cb71
Omar, A
4d7e34ce-ede1-4a87-9e37-9151ce4f5620
Peel, Kate
033a7ef7-a841-4b97-8bbc-be501315aae4
Provenzano, Giuseppe
076fb0cd-74db-4b62-bc0b-afffbe442cc4
Saleem, U
b6cd4615-3256-4704-86e0-9f3d47489252
Schmidt, Mark
19d14e64-2a68-41db-a067-375fb812b937
Schramm, Bettina
b0b1f7e9-0ba5-45db-a90d-e7b784d4befa
Sommer, S
845c4d42-0069-402a-8b10-e4ee41e8c6fa
Strong, James
0a6dc6d8-2a92-498b-b8a5-aa6d8f768008
Falcon Suarez, Ismael
2aca0a6e-fd1e-4ad9-a2cd-d98b13cd66d7
Ungerboeck, B
68661dae-12e1-45d2-9896-4aefef49fb5d
Widdicombe, Steve
3854c3ac-ad9d-4034-ba9e-1036047f88d8
Wright, H
faf4caff-13b3-4237-9c6c-74037eeec155
Yakushev, E
1b4d76af-357b-4205-b84b-6a7547e76e6b
Connelly, Douglas
a0d5c204-2cda-464a-850d-af1408d9de5f
Bull, Jonathan
974037fd-544b-458f-98cc-ce8eca89e3c8
Flohr, Anita
1e293a22-bdba-408e-9608-fed8b65e4e79
Koopmans, Dirk
abfee455-7f02-4de7-a4db-5b25cd7d8e03
Blackford, Jerry
0bd48334-2280-4209-aa74-8f411149b754
White, Paul
2dd2477b-5aa9-42e2-9d19-0806d994eaba
James, Rachael
79aa1d5c-675d-4ba3-85be-fb20798c02f4
Pearce, Chris
c8a35d08-42ce-46c7-82a6-7aba34890355
lichtschlag, Anna
56dc1ed4-7301-4e3f-9650-7c08162517cd
Achterberg, Eric
da742b45-3cf2-4ab4-8a51-1da00254c686
de Beer, Dirk
060ba2b9-7984-47b3-a206-c43f8b0fd110
Roche, Ben
08938cb1-4901-4f45-ba9a-aba53ed4ef7f
Li, Jianghui
9c589194-00fa-4d42-abaf-53a32789cc5e
Saw, Kevin
d17fe3b0-a61d-4ffc-bcf1-f24abd26e477
Alendal, G
f3063723-5b3d-4a38-adef-77a0663b0afc
Alvesen, H
0d510640-df81-4298-aa1a-4f14727db2df
Brown, R
aa3db44f-5ed8-475f-a28c-988031ff237e
Borisov, Sergei
6d842cf5-db81-440c-a6f4-c6831e020982
Bottner, Christoph
83baec2f-b6a6-4e0d-9e62-5da261de52fc
Cazenave, Pierre
869028e0-0c5d-4dc0-9e99-4d5b0d15747c
Chen, Baixin
001da024-c7b9-4629-a3d7-ccac1809d183
Dale, A
6c26d2d2-ff77-47bc-b962-60a7b861df1a
Dean, Marcella
561ef3e4-7234-4be5-bea8-396becfa247a
Dewar, Marius
5f898f03-2910-40ba-8b82-f6c755580657
Esposito, M
d87109c6-7315-46ac-b219-2a4c56870321
Gros, J
b6d6b05c-d170-46e3-9c39-b47bb1010687
Hanz, R
321f373e-7079-4afa-8954-fbf6ec88cf03
Haeckel, Matthias
dd9d005c-e484-4b57-a992-1d5cb7c3a3a7
Hosking, Brett
1d665df5-7c75-43c1-8b4a-ae4df5b8678c
Huvenne, veerle
2968611c-22f7-40ea-9e30-13ebf214b67b
Karstens, Jens
d87f50cb-dd8b-4b8f-85b0-3ad046642eb3
Le Bas, Tim
af315ced-85e0-4ec8-abfd-d80069685bb6
Leighton, Timothy
3e5262ce-1d7d-42eb-b013-fcc5c286bbae
Linke, Peter
f5865fb6-dbce-4072-8e6f-4fd313d0de71
Loucaides, S
9eeb8c5c-0212-4769-84b9-f860c9b96356
Matter, Juerg
abb60c24-b6cb-4d1a-a108-6fc51ee20395
Monk, S
4f47a781-581e-4dd0-aa58-4ec63e43776c
Mowlem, Matthew
ef893d5a-8244-4ab5-b605-11e0cac45b7a
Oleynik, A
55c41da0-c80c-46bc-916e-950c2cb0cb71
Omar, A
4d7e34ce-ede1-4a87-9e37-9151ce4f5620
Peel, Kate
033a7ef7-a841-4b97-8bbc-be501315aae4
Provenzano, Giuseppe
076fb0cd-74db-4b62-bc0b-afffbe442cc4
Saleem, U
b6cd4615-3256-4704-86e0-9f3d47489252
Schmidt, Mark
19d14e64-2a68-41db-a067-375fb812b937
Schramm, Bettina
b0b1f7e9-0ba5-45db-a90d-e7b784d4befa
Sommer, S
845c4d42-0069-402a-8b10-e4ee41e8c6fa
Strong, James
0a6dc6d8-2a92-498b-b8a5-aa6d8f768008
Falcon Suarez, Ismael
2aca0a6e-fd1e-4ad9-a2cd-d98b13cd66d7
Ungerboeck, B
68661dae-12e1-45d2-9896-4aefef49fb5d
Widdicombe, Steve
3854c3ac-ad9d-4034-ba9e-1036047f88d8
Wright, H
faf4caff-13b3-4237-9c6c-74037eeec155
Yakushev, E
1b4d76af-357b-4205-b84b-6a7547e76e6b

Connelly, Douglas, Bull, Jonathan, Flohr, Anita, Koopmans, Dirk, Blackford, Jerry, White, Paul, James, Rachael, Pearce, Chris, lichtschlag, Anna, Achterberg, Eric, de Beer, Dirk, Roche, Ben, Li, Jianghui, Saw, Kevin, Alendal, G, Alvesen, H, Brown, R, Borisov, Sergei, Bottner, Christoph, Cazenave, Pierre, Chen, Baixin, Dale, A, Dean, Marcella, Dewar, Marius, Esposito, M, Gros, J, Hanz, R, Haeckel, Matthias, Hosking, Brett, Huvenne, veerle, Karstens, Jens, Le Bas, Tim, Leighton, Timothy, Linke, Peter, Loucaides, S, Matter, Juerg, Monk, S, Mowlem, Matthew, Oleynik, A, Omar, A, Peel, Kate, Provenzano, Giuseppe, Saleem, U, Schmidt, Mark, Schramm, Bettina, Sommer, S, Strong, James, Falcon Suarez, Ismael, Ungerboeck, B, Widdicombe, Steve, Wright, H and Yakushev, E (2022) Assuring the integrity of offshore carbon dioxide storage. Renewable and Sustainable Energy Reviews, 166, [112670]. (doi:10.1016/j.rser.2022.112670).

Record type: Article

Abstract

Carbon capture and storage is a key mitigation strategy proposed for keeping the global temperature rise below 1.5 °C. Offshore storage can provide up to 13% of the global CO2 reduction required to achieve the Intergovernmental Panel on Climate Change goals. The public must be assured that potential leakages from storage reservoirs can be detected and that therefore the CO2 is safely contained. We conducted a controlled release of 675 kg CO2 within sediments at 120 m water depth, to simulate a leak and test novel detection, quantification and attribution approaches. We show that even at a very low release rate (6 kg day−1), CO2 can be detected within sediments and in the water column. Alongside detection we show the fluxes of both dissolved and gaseous CO2 can be quantified. The CO2 source was verified using natural and added tracers. The experiment demonstrates that existing technologies and techniques can detect, attribute and quantify any escape of CO2 from sub-seabed reservoirs as required for public assurance, regulatory oversight and emissions trading schemes.

Text
1-s2.0-S1364032122005627-main - Version of Record
Available under License Creative Commons Attribution.
Download (5MB)

More information

Accepted/In Press date: 2 June 2022
e-pub ahead of print date: 10 June 2022
Published date: September 2022
Additional Information: Funding Information: Funding was provided by the European Unions Horizon 2020 research and innovation programme under the grant agreement number 654462 (STEMM-CCS). We are grateful to the Captains and crews of the RRS James Cook and RV Poseidon for enabling the scientific measurements at sea during the JC180 and POS518, POS527, POS534 and MSM63 and MSM68 cruises. Mark Wells and the team at Cellular Robotics are thanked for the development of the seabed drilling system. We thank the support team at the National Marine Facilities at the NOC in Southampton for their unstinting help in the planning of the complex cruise programme. Publisher Copyright: © 2022 The Authors
Keywords: Carbon Capture and Storage, Carbon dioxide, MONITORING, Marine Carbon Capture and Storage, measurement, verification

Identifiers

Local EPrints ID: 467327
URI: http://eprints.soton.ac.uk/id/eprint/467327
ISSN: 1364-0321
PURE UUID: 0b74de5b-4e48-4529-90f6-640a726b3a09
ORCID for Jonathan Bull: ORCID iD orcid.org/0000-0003-3373-5807
ORCID for Anita Flohr: ORCID iD orcid.org/0000-0002-5018-5379
ORCID for Paul White: ORCID iD orcid.org/0000-0002-4787-8713
ORCID for Rachael James: ORCID iD orcid.org/0000-0001-7402-2315
ORCID for Ben Roche: ORCID iD orcid.org/0000-0002-0730-2947
ORCID for Jianghui Li: ORCID iD orcid.org/0000-0002-2956-5940
ORCID for Timothy Leighton: ORCID iD orcid.org/0000-0002-1649-8750
ORCID for Juerg Matter: ORCID iD orcid.org/0000-0002-1070-7371

Catalogue record

Date deposited: 06 Jul 2022 16:45
Last modified: 17 Mar 2024 03:30

Export record

Altmetrics

Contributors

Author: Douglas Connelly
Author: Jonathan Bull ORCID iD
Author: Anita Flohr ORCID iD
Author: Dirk Koopmans
Author: Jerry Blackford
Author: Paul White ORCID iD
Author: Rachael James ORCID iD
Author: Chris Pearce
Author: Anna lichtschlag
Author: Eric Achterberg
Author: Dirk de Beer
Author: Ben Roche ORCID iD
Author: Jianghui Li ORCID iD
Author: Kevin Saw
Author: G Alendal
Author: H Alvesen
Author: R Brown
Author: Sergei Borisov
Author: Christoph Bottner
Author: Pierre Cazenave
Author: Baixin Chen
Author: A Dale
Author: Marcella Dean
Author: Marius Dewar
Author: M Esposito
Author: J Gros
Author: R Hanz
Author: Matthias Haeckel
Author: Brett Hosking
Author: veerle Huvenne
Author: Jens Karstens
Author: Tim Le Bas
Author: Peter Linke
Author: S Loucaides
Author: Juerg Matter ORCID iD
Author: S Monk
Author: Matthew Mowlem
Author: A Oleynik
Author: A Omar
Author: Kate Peel
Author: Giuseppe Provenzano
Author: U Saleem
Author: Mark Schmidt
Author: Bettina Schramm
Author: S Sommer
Author: James Strong
Author: Ismael Falcon Suarez
Author: B Ungerboeck
Author: Steve Widdicombe
Author: H Wright
Author: E Yakushev

Download statistics

Downloads from ePrints over the past year. Other digital versions may also be available to download e.g. from the publisher's website.

View more statistics

Atom RSS 1.0 RSS 2.0

Contact ePrints Soton: eprints@soton.ac.uk

ePrints Soton supports OAI 2.0 with a base URL of http://eprints.soton.ac.uk/cgi/oai2

This repository has been built using EPrints software, developed at the University of Southampton, but available to everyone to use.

We use cookies to ensure that we give you the best experience on our website. If you continue without changing your settings, we will assume that you are happy to receive cookies on the University of Southampton website.

×