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How to measure χ(3) of a nanoparticle

How to measure χ(3) of a nanoparticle
How to measure χ(3) of a nanoparticle
Most of the known methods to measure the nonlinear optical properties of materials deal with the bulk properties, but there are many demanding applications that require those measurements to be done on a single particle or a single molecule. We report a novel application of nonlinear optics to measure the third-order nonlinear optical susceptibility of nanoparticles in solutions. By measuring the power of the third harmonic generated in a diluted solution of nanoparticles, both the size and χ(3) can be extracted from a simple set of measurements.
0146-9592
1486-1488
Shcheslavskiy, Vladislav I.
1e6126fc-61d7-49e1-a9be-826e10d117c1
Saltiel, Solomon M.
07ea07ba-79ed-4b07-a09c-57343d18d867
Faustov, Alexey R.
3e59a01e-0bc8-49fe-937d-aa104a2bf3c3
Petrov, Georgi I.
c8965815-6495-4263-aa4e-dc8f17352d8c
Yakovlev, Vladislav V.
aece8dee-ed5c-4a4b-b482-51e4fbea3963
Shcheslavskiy, Vladislav I.
1e6126fc-61d7-49e1-a9be-826e10d117c1
Saltiel, Solomon M.
07ea07ba-79ed-4b07-a09c-57343d18d867
Faustov, Alexey R.
3e59a01e-0bc8-49fe-937d-aa104a2bf3c3
Petrov, Georgi I.
c8965815-6495-4263-aa4e-dc8f17352d8c
Yakovlev, Vladislav V.
aece8dee-ed5c-4a4b-b482-51e4fbea3963

Shcheslavskiy, Vladislav I., Saltiel, Solomon M., Faustov, Alexey R., Petrov, Georgi I. and Yakovlev, Vladislav V. (2006) How to measure χ(3) of a nanoparticle. Optics Letters, 31 (10), 1486-1488. (doi:10.1364/OL.31.001486).

Record type: Article

Abstract

Most of the known methods to measure the nonlinear optical properties of materials deal with the bulk properties, but there are many demanding applications that require those measurements to be done on a single particle or a single molecule. We report a novel application of nonlinear optics to measure the third-order nonlinear optical susceptibility of nanoparticles in solutions. By measuring the power of the third harmonic generated in a diluted solution of nanoparticles, both the size and χ(3) can be extracted from a simple set of measurements.

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Published date: May 2006

Identifiers

Local EPrints ID: 46913
URI: http://eprints.soton.ac.uk/id/eprint/46913
ISSN: 0146-9592
PURE UUID: 2eb96ce8-1581-4476-88ec-00185a8e4ae3

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Date deposited: 24 Jul 2007
Last modified: 15 Mar 2024 09:28

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Contributors

Author: Vladislav I. Shcheslavskiy
Author: Solomon M. Saltiel
Author: Alexey R. Faustov
Author: Georgi I. Petrov
Author: Vladislav V. Yakovlev

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