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3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing

3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing
3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing
Memristors are emerging as promising candidates for practical application in reservoir computing systems that are capable of temporal information processing. Here, we experimentally implement a physical reservoir computing system using resistive memristors based on three-dimensional (3D)-structured mesoporous silica (mSiO2) thin films fabricated by a low cost, fast and vacuum-free sol–gel technique. The in situ learning capability and a classification accuracy of 100% on a standard machine learning dataset are experimentally demonstrated. The volatile (temporal) resistive switching in diffusive memristors arises from the formation and subsequent spontaneous rupture of conductive filaments via diffusion of Ag species within the 3D-structured nanopores of the mSiO2 thin film. Besides volatile switching, the devices also exhibit a bipolar non-volatile resistive switching behavior when the devices are operated at a higher compliance current level. The implementation of mSiO2 thin films opens the route to fabricate a simple and low cost dynamic memristor with a temporal information process functionality, which is essential for neuromorphic computing applications.
2040-3364
17170-17181
Hamdiyah, Ayoub Hassan Jaafar
ca3d9e21-e81e-491e-8a8a-b7b8f6e9fc84
Shao, Li
e273c42f-6065-40f8-8077-35a0b8a2505a
Dai, Peng
1150a00a-e54b-438b-bf51-4e8521c07f66
Zhang, Tongjun
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Han, Yisong
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Beanland, Richard
77643be6-0c38-4542-b05a-4ccc14efdc25
Kemp, Neil
6230af92-f8a5-4f73-8c23-1bd13ad15c7c
Bartlett, Philip N.
d99446db-a59d-4f89-96eb-f64b5d8bb075
Hector, Andrew L.
f19a8f31-b37f-4474-b32a-b7cf05b9f0e5
Huang, Ruomeng
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Hamdiyah, Ayoub Hassan Jaafar
ca3d9e21-e81e-491e-8a8a-b7b8f6e9fc84
Shao, Li
e273c42f-6065-40f8-8077-35a0b8a2505a
Dai, Peng
1150a00a-e54b-438b-bf51-4e8521c07f66
Zhang, Tongjun
4a460cd9-f2c8-41db-8008-1cda74895b24
Han, Yisong
9307e57c-85b5-461d-93c5-9c3081224c02
Beanland, Richard
77643be6-0c38-4542-b05a-4ccc14efdc25
Kemp, Neil
6230af92-f8a5-4f73-8c23-1bd13ad15c7c
Bartlett, Philip N.
d99446db-a59d-4f89-96eb-f64b5d8bb075
Hector, Andrew L.
f19a8f31-b37f-4474-b32a-b7cf05b9f0e5
Huang, Ruomeng
c6187811-ef2f-4437-8333-595c0d6ac978

Hamdiyah, Ayoub Hassan Jaafar, Shao, Li, Dai, Peng, Zhang, Tongjun, Han, Yisong, Beanland, Richard, Kemp, Neil, Bartlett, Philip N., Hector, Andrew L. and Huang, Ruomeng (2022) 3D-structured mesoporous silica memristors for neuromorphic switching and reservoir computing. Nanoscale, 14 (46), 17170-17181. (doi:10.1039/d2nr05012a).

Record type: Article

Abstract

Memristors are emerging as promising candidates for practical application in reservoir computing systems that are capable of temporal information processing. Here, we experimentally implement a physical reservoir computing system using resistive memristors based on three-dimensional (3D)-structured mesoporous silica (mSiO2) thin films fabricated by a low cost, fast and vacuum-free sol–gel technique. The in situ learning capability and a classification accuracy of 100% on a standard machine learning dataset are experimentally demonstrated. The volatile (temporal) resistive switching in diffusive memristors arises from the formation and subsequent spontaneous rupture of conductive filaments via diffusion of Ag species within the 3D-structured nanopores of the mSiO2 thin film. Besides volatile switching, the devices also exhibit a bipolar non-volatile resistive switching behavior when the devices are operated at a higher compliance current level. The implementation of mSiO2 thin films opens the route to fabricate a simple and low cost dynamic memristor with a temporal information process functionality, which is essential for neuromorphic computing applications.

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Accepted/In Press date: 10 November 2022
Published date: 10 November 2022

Identifiers

Local EPrints ID: 472949
URI: http://eprints.soton.ac.uk/id/eprint/472949
ISSN: 2040-3364
PURE UUID: 1c42fcc2-250d-49b1-bf11-f7d4dbf5b85d
ORCID for Ayoub Hassan Jaafar Hamdiyah: ORCID iD orcid.org/0000-0001-7305-4542
ORCID for Li Shao: ORCID iD orcid.org/0000-0001-6029-5574
ORCID for Peng Dai: ORCID iD orcid.org/0000-0002-5973-9155
ORCID for Philip N. Bartlett: ORCID iD orcid.org/0000-0002-7300-6900
ORCID for Andrew L. Hector: ORCID iD orcid.org/0000-0002-9964-2163
ORCID for Ruomeng Huang: ORCID iD orcid.org/0000-0003-1185-635X

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Date deposited: 06 Jan 2023 12:57
Last modified: 17 Mar 2024 04:12

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Contributors

Author: Ayoub Hassan Jaafar Hamdiyah ORCID iD
Author: Li Shao ORCID iD
Author: Peng Dai ORCID iD
Author: Tongjun Zhang
Author: Yisong Han
Author: Richard Beanland
Author: Neil Kemp
Author: Ruomeng Huang ORCID iD

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