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Hyperspectral visualization of picometric motion

Hyperspectral visualization of picometric motion
Hyperspectral visualization of picometric motion
The motion of nanostructures can be measured with picometric resolution using scattering of free electrons at sharp edges of the structures. Motion at the nano- to atomic scale is of growing technological importance and fundamental interest, in nano-electro-mechanical systems (NEMS), advanced materials (e.g. nanowires, 2D materials), mechanically reconfigurable photonic metamaterials; and in the study of systems governed by Van der Waals and Casimir forces, and quantum phenomena. However, there are no routinely available technologies for quantifying and spatially mapping fast, complex movements of picometric amplitude in nanostructures. We show how the spectrallyresolved detection of scattering from a tightly-focused free-electron beam incident on the sharp edges of a nano-object can provide for quantitative 3D visualization of motion at the picoscale. For a range of nano/microstructures, from simple cantilevers to photonic metamaterials and MEMS comb-drive actuators, we demonstrate measurements of thermal (cf. Brownian) motion amplitudes down to a noise-equivalent displacement level of 1 pm/Hz1/2, and the mapping of driven-motion oscillatory ‘mode shapes’ with spatial (SEM imaging) resolution far beyond the diffraction limit applicable to optical vibrometry techniques.
We also report on the first observation of short-timescale ‘ballistic’ thermal motion in the flexural mode of a nanomembrane cantilever, driven by thermal fluctuation of flexural phonon numbers in the membrane: over intervals <10 μs, the membrane is found to move ballistically, at an average constant velocity of ~300 μm/s, while Brownian-like dynamics emerge for longer observation times. Access to the ballistic regime provides verification of the equipartition theorem and Maxwell-Boltzmann statistics for flexural modes and presents opportunities in fast thermometry and mass sensing.
MacDonald, Kevin F.
76c84116-aad1-4973-b917-7ca63935dba5
Liu, Tongjun
53eb4a71-ea7b-4aa7-b96d-b70c5df1dd63
Ou, Jun-Yu
3fb703e3-b222-46d2-b4ee-75f296d9d64d
Zheludev, Nikolai
32fb6af7-97e4-4d11-bca6-805745e40cc6
MacDonald, Kevin F.
76c84116-aad1-4973-b917-7ca63935dba5
Liu, Tongjun
53eb4a71-ea7b-4aa7-b96d-b70c5df1dd63
Ou, Jun-Yu
3fb703e3-b222-46d2-b4ee-75f296d9d64d
Zheludev, Nikolai
32fb6af7-97e4-4d11-bca6-805745e40cc6

MacDonald, Kevin F., Liu, Tongjun, Ou, Jun-Yu and Zheludev, Nikolai (2023) Hyperspectral visualization of picometric motion. Microscopy Conference 2023, , Darmstadt, Germany. 26 Feb - 02 Mar 2023. 1 pp .

Record type: Conference or Workshop Item (Paper)

Abstract

The motion of nanostructures can be measured with picometric resolution using scattering of free electrons at sharp edges of the structures. Motion at the nano- to atomic scale is of growing technological importance and fundamental interest, in nano-electro-mechanical systems (NEMS), advanced materials (e.g. nanowires, 2D materials), mechanically reconfigurable photonic metamaterials; and in the study of systems governed by Van der Waals and Casimir forces, and quantum phenomena. However, there are no routinely available technologies for quantifying and spatially mapping fast, complex movements of picometric amplitude in nanostructures. We show how the spectrallyresolved detection of scattering from a tightly-focused free-electron beam incident on the sharp edges of a nano-object can provide for quantitative 3D visualization of motion at the picoscale. For a range of nano/microstructures, from simple cantilevers to photonic metamaterials and MEMS comb-drive actuators, we demonstrate measurements of thermal (cf. Brownian) motion amplitudes down to a noise-equivalent displacement level of 1 pm/Hz1/2, and the mapping of driven-motion oscillatory ‘mode shapes’ with spatial (SEM imaging) resolution far beyond the diffraction limit applicable to optical vibrometry techniques.
We also report on the first observation of short-timescale ‘ballistic’ thermal motion in the flexural mode of a nanomembrane cantilever, driven by thermal fluctuation of flexural phonon numbers in the membrane: over intervals <10 μs, the membrane is found to move ballistically, at an average constant velocity of ~300 μm/s, while Brownian-like dynamics emerge for longer observation times. Access to the ballistic regime provides verification of the equipartition theorem and Maxwell-Boltzmann statistics for flexural modes and presents opportunities in fast thermometry and mass sensing.

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MC23 SEM motion visualization - Accepted Manuscript
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Published date: 26 February 2023
Venue - Dates: Microscopy Conference 2023, , Darmstadt, Germany, 2023-02-26 - 2023-03-02

Identifiers

Local EPrints ID: 474078
URI: http://eprints.soton.ac.uk/id/eprint/474078
PURE UUID: 304d728a-bd4f-43ee-bdfa-423829c34492
ORCID for Kevin F. MacDonald: ORCID iD orcid.org/0000-0002-3877-2976
ORCID for Jun-Yu Ou: ORCID iD orcid.org/0000-0001-8028-6130
ORCID for Nikolai Zheludev: ORCID iD orcid.org/0000-0002-1013-6636

Catalogue record

Date deposited: 10 Feb 2023 17:56
Last modified: 17 Mar 2024 07:38

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Contributors

Author: Tongjun Liu
Author: Jun-Yu Ou ORCID iD

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