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A review on mathematical modelling of direct internal reforming- solid oxide fuel cells

A review on mathematical modelling of direct internal reforming- solid oxide fuel cells
A review on mathematical modelling of direct internal reforming- solid oxide fuel cells
The Solid Oxide Fuel Cells (SOFCs) anode materials are catalytically active for Direct Internal Reforming (DIR) thus avoiding the need of external reformer. However, practical application of DIR in SOFCs requires careful system design and selection of operating conditions to avoid cell degradation due to carbon depositions and other impurities. In recent years, numerous simulation studies, besides experimental investigations, have been carried out to understand the physical and electrochemical complexities of DIR-based SOFC systems in order to develop viable designs and optimize the operating conditions before conducting costly experiments. The objective of this work is to review the present status of DIR-SOFC modeling efforts and consolidate their findings in order to highlight the unresolved problems for future research in this field. A specific focus of this review has been given to the multiscale mathematical modeling. Pre-reforming techniques, influences of the chemical and electrochemical reaction kinetics and operational variables along with future prospects of the DIR-SOFC have been also reviewed and discussed.
0378-7753
Faheem, Hafiz Hamza
39610ff5-be98-4403-a5fd-3fdbc5f75cac
Abbas, Syed Zaheer
3b02900e-fef6-40e1-acf7-96f26bfde4a8
Tabish, Asif Nadeem
ae1a81ab-39b3-4f5f-aa3e-c8e228c7998a
Fan, Liyuan
6d31707e-7d87-4923-8c6a-5ff5e6165d93
Maqbool, Fahad
608013cc-6fab-45dd-b848-9f42e796bf10
Faheem, Hafiz Hamza
39610ff5-be98-4403-a5fd-3fdbc5f75cac
Abbas, Syed Zaheer
3b02900e-fef6-40e1-acf7-96f26bfde4a8
Tabish, Asif Nadeem
ae1a81ab-39b3-4f5f-aa3e-c8e228c7998a
Fan, Liyuan
6d31707e-7d87-4923-8c6a-5ff5e6165d93
Maqbool, Fahad
608013cc-6fab-45dd-b848-9f42e796bf10

Faheem, Hafiz Hamza, Abbas, Syed Zaheer, Tabish, Asif Nadeem, Fan, Liyuan and Maqbool, Fahad (2021) A review on mathematical modelling of direct internal reforming- solid oxide fuel cells. Journal of Power Sources, 520, [230857]. (doi:10.1016/j.jpowsour.2021.230857).

Record type: Article

Abstract

The Solid Oxide Fuel Cells (SOFCs) anode materials are catalytically active for Direct Internal Reforming (DIR) thus avoiding the need of external reformer. However, practical application of DIR in SOFCs requires careful system design and selection of operating conditions to avoid cell degradation due to carbon depositions and other impurities. In recent years, numerous simulation studies, besides experimental investigations, have been carried out to understand the physical and electrochemical complexities of DIR-based SOFC systems in order to develop viable designs and optimize the operating conditions before conducting costly experiments. The objective of this work is to review the present status of DIR-SOFC modeling efforts and consolidate their findings in order to highlight the unresolved problems for future research in this field. A specific focus of this review has been given to the multiscale mathematical modeling. Pre-reforming techniques, influences of the chemical and electrochemical reaction kinetics and operational variables along with future prospects of the DIR-SOFC have been also reviewed and discussed.

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Accepted/In Press date: 29 November 2021
e-pub ahead of print date: 13 December 2021

Identifiers

Local EPrints ID: 474416
URI: http://eprints.soton.ac.uk/id/eprint/474416
ISSN: 0378-7753
PURE UUID: 29ce7814-2c1b-40f5-9d55-a16fcf18ad02
ORCID for Syed Zaheer Abbas: ORCID iD orcid.org/0000-0002-8783-8572

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Date deposited: 21 Feb 2023 17:56
Last modified: 17 Mar 2024 04:18

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Contributors

Author: Hafiz Hamza Faheem
Author: Syed Zaheer Abbas ORCID iD
Author: Asif Nadeem Tabish
Author: Liyuan Fan
Author: Fahad Maqbool

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