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Removal of benzene as a tar model compound from a gas mixture using non-thermal plasma dielectric barrier discharge reactor

Removal of benzene as a tar model compound from a gas mixture using non-thermal plasma dielectric barrier discharge reactor
Removal of benzene as a tar model compound from a gas mixture using non-thermal plasma dielectric barrier discharge reactor
In the present work, the decomposition of benzene as a tar model compound was studied in a gas mixture (CO2, H2, CO, and CH4) using a dielectric barrier discharge (DBD) non-thermal plasma reactor. The combined effect of temperature and power was studied to investigate the performance of the DBD reactor. The decomposition of tar compound increased from 49.9 to 96% with increasing specific input energy (SIE) from 2.05 to 16.4 kWh/m3. The major products were lower hydrocarbons (C2–C5) and solid residues. The higher temperature (400 °C) in the presence of plasma (40 W), decreased the conversion of tar compound from 96 to 78%. However, the selectivity of lower hydrocarbons increases substantially to 52%, and the formation of solid residues is significantly reduced. Hence, the problematic solid residues formation can be controlled at a higher temperature during the treatment of gasifier product gas using non-thermal plasma.
1743-9671
97-105
Saleem, Faisal
f13d5fc2-1bca-4506-9ab9-866e4d0f996d
Hussain Khoja, Asif
2407c353-337d-4c27-a42d-a0816bb909eb
Umer, Jamal
21690c1f-df1f-4418-afcd-d480770befc2
Ahmad, Farhan
31d3a50a-a198-40ae-abc2-d5c8735bcc3c
Abbas, Syed Zaheer
3b02900e-fef6-40e1-acf7-96f26bfde4a8
Zhang, Kui
50ad16d2-f782-4575-aa87-3acd79b51714
Harvey, Adam
ea612d8a-f0ff-4c7c-a42a-dc0f0bcbabbd
Saleem, Faisal
f13d5fc2-1bca-4506-9ab9-866e4d0f996d
Hussain Khoja, Asif
2407c353-337d-4c27-a42d-a0816bb909eb
Umer, Jamal
21690c1f-df1f-4418-afcd-d480770befc2
Ahmad, Farhan
31d3a50a-a198-40ae-abc2-d5c8735bcc3c
Abbas, Syed Zaheer
3b02900e-fef6-40e1-acf7-96f26bfde4a8
Zhang, Kui
50ad16d2-f782-4575-aa87-3acd79b51714
Harvey, Adam
ea612d8a-f0ff-4c7c-a42a-dc0f0bcbabbd

Saleem, Faisal, Hussain Khoja, Asif, Umer, Jamal, Ahmad, Farhan, Abbas, Syed Zaheer, Zhang, Kui and Harvey, Adam (2021) Removal of benzene as a tar model compound from a gas mixture using non-thermal plasma dielectric barrier discharge reactor. Journal of the Energy Institute, 96, 97-105. (doi:10.1016/j.joei.2021.02.008).

Record type: Article

Abstract

In the present work, the decomposition of benzene as a tar model compound was studied in a gas mixture (CO2, H2, CO, and CH4) using a dielectric barrier discharge (DBD) non-thermal plasma reactor. The combined effect of temperature and power was studied to investigate the performance of the DBD reactor. The decomposition of tar compound increased from 49.9 to 96% with increasing specific input energy (SIE) from 2.05 to 16.4 kWh/m3. The major products were lower hydrocarbons (C2–C5) and solid residues. The higher temperature (400 °C) in the presence of plasma (40 W), decreased the conversion of tar compound from 96 to 78%. However, the selectivity of lower hydrocarbons increases substantially to 52%, and the formation of solid residues is significantly reduced. Hence, the problematic solid residues formation can be controlled at a higher temperature during the treatment of gasifier product gas using non-thermal plasma.

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Accepted/In Press date: 23 February 2021
e-pub ahead of print date: 27 February 2021
Published date: 10 March 2021

Identifiers

Local EPrints ID: 475068
URI: http://eprints.soton.ac.uk/id/eprint/475068
ISSN: 1743-9671
PURE UUID: 9b94fb59-dc57-4bbf-8787-e232ef92f5e9
ORCID for Syed Zaheer Abbas: ORCID iD orcid.org/0000-0002-8783-8572

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Date deposited: 09 Mar 2023 19:02
Last modified: 17 Mar 2024 04:18

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Contributors

Author: Faisal Saleem
Author: Asif Hussain Khoja
Author: Jamal Umer
Author: Farhan Ahmad
Author: Syed Zaheer Abbas ORCID iD
Author: Kui Zhang
Author: Adam Harvey

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