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Unsaturated flow and solute transport through the Chalk: tracer test and dual permeability modelling

Unsaturated flow and solute transport through the Chalk: tracer test and dual permeability modelling
Unsaturated flow and solute transport through the Chalk: tracer test and dual permeability modelling
A tracer test was carried out in the unsaturated Chalk at the Fleam Dyke research site in Cambridgeshire, UK, to investigate the role of the Chalk fractures and matrix in unsaturated flow and solute transport. The experiment, under natural rainfall conditions, involved distributing deuterated water on a grass-covered lysimeter (a cube of volume 125 m3) and on an adjacent 4 m × 4 m field plot. Tracer migration was monitored through regular core sampling and collection of lysimeter drainage water. The presence of occasional secondary peaks in sampling of the vertical tracer profile suggested the occurrence of fracture flow, allowing some tracer to bypass the Chalk matrix. However, in the 15 months following application, none of the tracer was detected in the lysimeter drainage at 5 m depth. Modelling of the tracer results was undertaken with the 1-D numerical transient dual permeability model MACRO 5.0, initially developed for macroporous soils. Modelling results showed that MACRO 5.0 could reliably simulate transient recharge through the Chalk. The simulations suggested that fracture flow is important at the site, but that it is only initiated at 1 m depth or deeper. The extent of fracture flow appeared to be highly variable in different layers of the profile, varying between 40% and 85% of the cumulative flux, mainly depending on the saturated hydraulic conductivity of the matrix. Diffusion between the fractures and the matrix tended to equalize solute concentrations in both flow domains, although solute bypass through the fractures occurred in some Chalk strata. Besides diffusive exchange, the modelling stressed the importance of advective exchange of solutes. The results suggest that the Chalk aquifer at the Fleam Dyke site is only moderately vulnerable to pollution, even though for moderate rainfall conditions some bypass flow was possible.
Chalk, dual permeability models, tracer test, matrix diffusion, unsaturated zone
0022-1694
157-172
Van den Daele, Gerd F.A.
7f057f48-34da-45da-a7d7-c9f85057c085
Barker, John A.
33bf9dec-cc9b-451c-8192-46099e316b6d
Connell, Luke D.
2b40d1b3-f5e1-484d-aa46-ec792c8db870
Atkinson, Tim C.
8c472a13-2711-49c7-aa7d-f44869e201ab
Darling, W.G.
5148f637-7437-4b8e-a7a9-72e285178c52
Cooper, J.D.
d3363e20-4ea6-46cf-82c7-d8812d5787c6
Van den Daele, Gerd F.A.
7f057f48-34da-45da-a7d7-c9f85057c085
Barker, John A.
33bf9dec-cc9b-451c-8192-46099e316b6d
Connell, Luke D.
2b40d1b3-f5e1-484d-aa46-ec792c8db870
Atkinson, Tim C.
8c472a13-2711-49c7-aa7d-f44869e201ab
Darling, W.G.
5148f637-7437-4b8e-a7a9-72e285178c52
Cooper, J.D.
d3363e20-4ea6-46cf-82c7-d8812d5787c6

Van den Daele, Gerd F.A., Barker, John A., Connell, Luke D., Atkinson, Tim C., Darling, W.G. and Cooper, J.D. (2007) Unsaturated flow and solute transport through the Chalk: tracer test and dual permeability modelling. Journal of Hydrology, 342 (1-2), 157-172. (doi:10.1016/j.jhydrol.2007.05.021).

Record type: Article

Abstract

A tracer test was carried out in the unsaturated Chalk at the Fleam Dyke research site in Cambridgeshire, UK, to investigate the role of the Chalk fractures and matrix in unsaturated flow and solute transport. The experiment, under natural rainfall conditions, involved distributing deuterated water on a grass-covered lysimeter (a cube of volume 125 m3) and on an adjacent 4 m × 4 m field plot. Tracer migration was monitored through regular core sampling and collection of lysimeter drainage water. The presence of occasional secondary peaks in sampling of the vertical tracer profile suggested the occurrence of fracture flow, allowing some tracer to bypass the Chalk matrix. However, in the 15 months following application, none of the tracer was detected in the lysimeter drainage at 5 m depth. Modelling of the tracer results was undertaken with the 1-D numerical transient dual permeability model MACRO 5.0, initially developed for macroporous soils. Modelling results showed that MACRO 5.0 could reliably simulate transient recharge through the Chalk. The simulations suggested that fracture flow is important at the site, but that it is only initiated at 1 m depth or deeper. The extent of fracture flow appeared to be highly variable in different layers of the profile, varying between 40% and 85% of the cumulative flux, mainly depending on the saturated hydraulic conductivity of the matrix. Diffusion between the fractures and the matrix tended to equalize solute concentrations in both flow domains, although solute bypass through the fractures occurred in some Chalk strata. Besides diffusive exchange, the modelling stressed the importance of advective exchange of solutes. The results suggest that the Chalk aquifer at the Fleam Dyke site is only moderately vulnerable to pollution, even though for moderate rainfall conditions some bypass flow was possible.

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More information

Submitted date: 11 February 2007
Published date: 15 August 2007
Additional Information: Received 11 February 2007; revised 19 May 2007; accepted 23 May 2007.
Keywords: Chalk, dual permeability models, tracer test, matrix diffusion, unsaturated zone
Organisations: Civil Engineering & the Environment

Identifiers

Local EPrints ID: 48128
URI: http://eprints.soton.ac.uk/id/eprint/48128
ISSN: 0022-1694
PURE UUID: 76f4924e-e8f4-434b-92fe-9f31aa637ea4

Catalogue record

Date deposited: 29 Aug 2007
Last modified: 15 Mar 2024 09:43

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Contributors

Author: Gerd F.A. Van den Daele
Author: John A. Barker
Author: Luke D. Connell
Author: Tim C. Atkinson
Author: W.G. Darling
Author: J.D. Cooper

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