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A CFD study of biomass pyrolysis in a downer reactor equipped with a novel gas-solid separator-II thermochemical performance and products

A CFD study of biomass pyrolysis in a downer reactor equipped with a novel gas-solid separator-II thermochemical performance and products
A CFD study of biomass pyrolysis in a downer reactor equipped with a novel gas-solid separator-II thermochemical performance and products

A Eulerian-Eulerian CFD model was used to investigate the fast pyrolysis of biomass in a downer reactor equipped with a novel gas-solid separation mechanism. The highly endothermic pyrolysis reaction was assumed to be entirely driven by an inert solid heat carrier (sand). A one-step global pyrolysis reaction, along with the equations describing the biomass drying and heat transfer, was implemented in the hydrodynamic model presented in part I of this study (Fuel Processing Technology, V126, 366-382). The predictions of the gas-solid separation efficiency, temperature distribution, residence time and the pyrolysis product yield are presented and discussed. For the operating conditions considered, the devolatilisation efficiency was found to be above 60% and the yield composition in mass fraction was 56.85% bio-oil, 37.87% bio-char and 5.28% non-condensable gas (NCG). This has been found to agree reasonably well with recent relevant published experimental data. The novel gas-solid separation mechanism allowed achieving greater than 99.9% separation efficiency and < 2 s pyrolysis gas residence time. The model has been found to be robust and fast in terms of computational time, thus has the great potential to aid in future design and optimisation of the biomass fast pyrolysis process.

Biomass, CFD modeling, Downer reactor, Fast pyrolysis
0378-3820
51-63
Yu, Xi
7e4f553f-cc11-4c6e-ad6d-9fb5c3c07a60
Hassan, Mohamed
ce323212-f178-4d72-85cf-23cd30605cd8
Ocone, Raffaella
89db17bd-1848-4c75-ac00-40b9c077b1a8
Makkawi, Yassir
217bdad4-a83f-44a9-ab54-b52633298456
Yu, Xi
7e4f553f-cc11-4c6e-ad6d-9fb5c3c07a60
Hassan, Mohamed
ce323212-f178-4d72-85cf-23cd30605cd8
Ocone, Raffaella
89db17bd-1848-4c75-ac00-40b9c077b1a8
Makkawi, Yassir
217bdad4-a83f-44a9-ab54-b52633298456

Yu, Xi, Hassan, Mohamed, Ocone, Raffaella and Makkawi, Yassir (2015) A CFD study of biomass pyrolysis in a downer reactor equipped with a novel gas-solid separator-II thermochemical performance and products. Fuel Processing Technology, 133, 51-63. (doi:10.1016/j.fuproc.2015.01.002).

Record type: Article

Abstract

A Eulerian-Eulerian CFD model was used to investigate the fast pyrolysis of biomass in a downer reactor equipped with a novel gas-solid separation mechanism. The highly endothermic pyrolysis reaction was assumed to be entirely driven by an inert solid heat carrier (sand). A one-step global pyrolysis reaction, along with the equations describing the biomass drying and heat transfer, was implemented in the hydrodynamic model presented in part I of this study (Fuel Processing Technology, V126, 366-382). The predictions of the gas-solid separation efficiency, temperature distribution, residence time and the pyrolysis product yield are presented and discussed. For the operating conditions considered, the devolatilisation efficiency was found to be above 60% and the yield composition in mass fraction was 56.85% bio-oil, 37.87% bio-char and 5.28% non-condensable gas (NCG). This has been found to agree reasonably well with recent relevant published experimental data. The novel gas-solid separation mechanism allowed achieving greater than 99.9% separation efficiency and < 2 s pyrolysis gas residence time. The model has been found to be robust and fast in terms of computational time, thus has the great potential to aid in future design and optimisation of the biomass fast pyrolysis process.

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More information

Published date: May 2015
Keywords: Biomass, CFD modeling, Downer reactor, Fast pyrolysis

Identifiers

Local EPrints ID: 481488
URI: http://eprints.soton.ac.uk/id/eprint/481488
ISSN: 0378-3820
PURE UUID: f94692e6-6442-4620-a601-480601821567
ORCID for Mohamed Hassan: ORCID iD orcid.org/0000-0003-3729-4543

Catalogue record

Date deposited: 30 Aug 2023 16:34
Last modified: 06 Jun 2024 02:19

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Contributors

Author: Xi Yu ORCID iD
Author: Mohamed Hassan ORCID iD
Author: Raffaella Ocone
Author: Yassir Makkawi

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