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Synergistic overview and perspectives of two-dimensional heterostructures for cathodes and separators in flexible Li–S batteries

Synergistic overview and perspectives of two-dimensional heterostructures for cathodes and separators in flexible Li–S batteries
Synergistic overview and perspectives of two-dimensional heterostructures for cathodes and separators in flexible Li–S batteries
Because of their high energy densities and specific capacities, lithium–sulfur (Li–S) batteries have recently received an extensive amount of research. The best way to boost battery performance is by altering the electrode materials. The adoption of 2D material-based heterostructures has attracted significant attention for increasing electrochemical performance and preventing the shuttle effect. Therefore, a summary of the link between the specific properties of 2D material heterostructures and electrochemical performance is required for the development of next-generation Li–S batteries. The present research focuses on the latest developments that boost the performance of Li–S batteries by using the unique features of 2D material heterostructures. This evaluation also categorizes several meticulously selected 2D materials with specific properties. Some solutions have been developed to overcome the difficulties of insulating intermediates, polysulfide shuttle, and sluggish kinetics. Superior conductivity, tunable functional groups, and exceptional flexibility are some of the most crucial elements in boosting electrochemical performance.
0887-0624
10827–10842
Kiai, Maryam Sadat
c0c83cdd-42e4-4e61-9150-9c40071e2000
Ponnada, Srikanth
269dcc54-70d2-4b0b-9bc6-0e81ad066c07
Mansoor, Mubashir
5a5f2503-4b07-426f-87d3-bc5859179f8c
Aslfattahi, Navid
f757925a-2306-4e33-9489-b34bc6a7b501
Naskar, Susmita
5f787953-b062-4774-a28b-473bd19254b1
Kiai, Maryam Sadat
c0c83cdd-42e4-4e61-9150-9c40071e2000
Ponnada, Srikanth
269dcc54-70d2-4b0b-9bc6-0e81ad066c07
Mansoor, Mubashir
5a5f2503-4b07-426f-87d3-bc5859179f8c
Aslfattahi, Navid
f757925a-2306-4e33-9489-b34bc6a7b501
Naskar, Susmita
5f787953-b062-4774-a28b-473bd19254b1

Kiai, Maryam Sadat, Ponnada, Srikanth, Mansoor, Mubashir, Aslfattahi, Navid and Naskar, Susmita (2023) Synergistic overview and perspectives of two-dimensional heterostructures for cathodes and separators in flexible Li–S batteries. Energy & Fuels, 37 (15), 10827–10842. (doi:10.1021/acs.energyfuels.3c01410).

Record type: Review

Abstract

Because of their high energy densities and specific capacities, lithium–sulfur (Li–S) batteries have recently received an extensive amount of research. The best way to boost battery performance is by altering the electrode materials. The adoption of 2D material-based heterostructures has attracted significant attention for increasing electrochemical performance and preventing the shuttle effect. Therefore, a summary of the link between the specific properties of 2D material heterostructures and electrochemical performance is required for the development of next-generation Li–S batteries. The present research focuses on the latest developments that boost the performance of Li–S batteries by using the unique features of 2D material heterostructures. This evaluation also categorizes several meticulously selected 2D materials with specific properties. Some solutions have been developed to overcome the difficulties of insulating intermediates, polysulfide shuttle, and sluggish kinetics. Superior conductivity, tunable functional groups, and exceptional flexibility are some of the most crucial elements in boosting electrochemical performance.

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ef-2023-01410a.R2_Proof_hi - Accepted Manuscript
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More information

e-pub ahead of print date: 25 July 2023
Published date: 3 August 2023
Additional Information: Funding Information: All authors would like to thank University College of Dublin-Ireland, Indian Institute of Technology Jodhpur-India, Czech Technical University in Prague, and University of Southampton-United Kingdom for resource and technical support. Publisher Copyright: © 2023 American Chemical Society.

Identifiers

Local EPrints ID: 484651
URI: http://eprints.soton.ac.uk/id/eprint/484651
ISSN: 0887-0624
PURE UUID: 92d7af08-9a1e-4b7a-9cf0-665530a33f16
ORCID for Susmita Naskar: ORCID iD orcid.org/0000-0003-3294-8333

Catalogue record

Date deposited: 20 Nov 2023 17:32
Last modified: 03 Aug 2024 04:01

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Contributors

Author: Maryam Sadat Kiai
Author: Srikanth Ponnada
Author: Mubashir Mansoor
Author: Navid Aslfattahi
Author: Susmita Naskar ORCID iD

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