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Cathodes for electrochemical carbon dioxide reduction to multi-carbon products: part I : a focused review of recent highlights

Cathodes for electrochemical carbon dioxide reduction to multi-carbon products: part I : a focused review of recent highlights
Cathodes for electrochemical carbon dioxide reduction to multi-carbon products: part I : a focused review of recent highlights
This is a focused review of recent highlights in the literature in cathode development for low temperature electrochemical carbon dioxide and carbon monoxide reduction to multi-carbon (C2+) products. The major goals for the field are to increase Faradaic efficiency (FE) for specific C2+ products, lower cell voltage for industrially relevant current densities and increase cell lifetime. A key to achieving these goals is the rational design of cathodes through increased understanding of structure-selectivity and structure-activity relationships for catalysts and the influence of catalyst binders and gas diffusion layers (GDLs) on the catalyst microenvironment and subsequent performance.
97-109
Macpherson, Harry
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Hodges, Toby
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Chuma, Moyahabo Hellen
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Sherwin, Connor
b4e01340-ac4d-46a3-8904-ec306c903761
Podbevšek, Urša
ffcc80dc-5dd8-4c8a-81e1-80da87a6b128
Rigg, Katie
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Celorrio, Veronica
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Russell, Andrea
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Corbos, Elena C.
fb2d9cfb-e361-471f-8d05-f07ba67aa669
Macpherson, Harry
3826727a-471c-4266-a9cd-23f88d1a3d6a
Hodges, Toby
a60b0292-f3b7-4e31-9d17-05b8f0bb00ff
Chuma, Moyahabo Hellen
d61d282e-dd96-4ce8-8aa0-b27da05bac5f
Sherwin, Connor
b4e01340-ac4d-46a3-8904-ec306c903761
Podbevšek, Urša
ffcc80dc-5dd8-4c8a-81e1-80da87a6b128
Rigg, Katie
2051cc16-6c45-4808-be02-be4281f29f17
Celorrio, Veronica
5ebb7fb5-a74c-4872-9795-5830dc915d0b
Russell, Andrea
b6b7c748-efc1-4d5d-8a7a-8e4b69396169
Corbos, Elena C.
fb2d9cfb-e361-471f-8d05-f07ba67aa669

Macpherson, Harry, Hodges, Toby, Chuma, Moyahabo Hellen, Sherwin, Connor, Podbevšek, Urša, Rigg, Katie, Celorrio, Veronica, Russell, Andrea and Corbos, Elena C. (2022) Cathodes for electrochemical carbon dioxide reduction to multi-carbon products: part I : a focused review of recent highlights. Johnson Matthey Technology Review, 67 (1), 97-109. (doi:10.1595/205651323x16672291226135).

Record type: Article

Abstract

This is a focused review of recent highlights in the literature in cathode development for low temperature electrochemical carbon dioxide and carbon monoxide reduction to multi-carbon (C2+) products. The major goals for the field are to increase Faradaic efficiency (FE) for specific C2+ products, lower cell voltage for industrially relevant current densities and increase cell lifetime. A key to achieving these goals is the rational design of cathodes through increased understanding of structure-selectivity and structure-activity relationships for catalysts and the influence of catalyst binders and gas diffusion layers (GDLs) on the catalyst microenvironment and subsequent performance.

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Accepted/In Press date: 27 October 2022
e-pub ahead of print date: 31 October 2022

Identifiers

Local EPrints ID: 491885
URI: http://eprints.soton.ac.uk/id/eprint/491885
PURE UUID: ca7517a1-f295-454a-83ed-7f3c44d02a5e
ORCID for Connor Sherwin: ORCID iD orcid.org/0000-0002-2710-5991
ORCID for Andrea Russell: ORCID iD orcid.org/0000-0002-8382-6443

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Date deposited: 04 Jul 2024 18:12
Last modified: 12 Jul 2024 02:07

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Contributors

Author: Harry Macpherson
Author: Toby Hodges
Author: Moyahabo Hellen Chuma
Author: Connor Sherwin ORCID iD
Author: Urša Podbevšek
Author: Katie Rigg
Author: Veronica Celorrio
Author: Andrea Russell ORCID iD
Author: Elena C. Corbos

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