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Associations of cord plasma per- and polyfluoroakyl substances (PFAS) with neonatal and child body composition and adiposity: the GUSTO study

Associations of cord plasma per- and polyfluoroakyl substances (PFAS) with neonatal and child body composition and adiposity: the GUSTO study
Associations of cord plasma per- and polyfluoroakyl substances (PFAS) with neonatal and child body composition and adiposity: the GUSTO study

Background: the influence of prenatal exposure to per- and poly- fluoroalkyl substances (PFAS) on birth size and offspring adiposity is unclear, especially for the newer, shorter-chained replacement PFAS. 

Methods: in the GUSTO multi-ethnic Singaporean mother-offspring cohort, 12 PFAS were measured in 783 cord plasma samples using ultra-performance-liquid chromatography-tandem-mass-spectrometer (UPLC-MS/MS). Outcomes included offspring anthropometry, other indicators of body composition/metabolic health, and MRI-derived abdominal adiposity (subset) at birth and 6 years of age. PFAS were modeled individually, in categories of long-chain and short-chain PFAS, and as scores of three principal components (PC) derived using PC analysis (PC1, PC2, and PC3 reflect predominant exposure patterns to “very-long-PFAS”, “long-PFAS”, and “short-PFAS”, respectively). Associations with outcomes were assessed using multivariable linear regressions, adjusted for important covariates such as maternal sociodemographic and lifestyle factors. 

Results: overall, cord PFAS levels showed either no or positive associations (mostly for long-chain PFAS) with birth weight, length and head circumference. In general, PFAS were associated with higher neonatal abdominal adiposity, driven by shorter-chain PFAS. Perfluoroheptanoic acid (PFHpA) was associated with higher volumes of superficial subcutaneous adipose tissue (sSAT) (3.75 [1.13, 6.37] mL per SD increase in PFAS) and internal adipose tissue (IAT) (1.39 [0.41, 2.38] mL). Higher levels of perfluorobutanesulfonic acid (PFBS), short-chain PFAS, and PC3 were associated with higher IAT volume (β range 1.22–1.41 mL/SD, all P < 0.02), especially in girls. Higher PC3 score was additionally associated with higher sSAT (3.12 [0.45, 5.80] mL) volume. At age 6 years, most observed associations did not persist. No consistent associations were observed between PFAS and whole-body adiposity measures. 

Conclusions: fetal exposure to emerging short-chain PFAS was associated with higher abdominal adiposity at birth but not at age 6 years. Further research is needed to replicate the findings and to determine if these effects may reappear beyond early childhood. Population exposure to newer PFAS and consequent health impact must be monitored.

Adiposity, Alkanesulfonic Acids, Body Composition, Child, Child, Preschool, Chromatography, Liquid, Environmental Pollutants, Female, Fluorocarbons, Humans, Infant, Newborn, Obesity, Obesity, Abdominal, Pregnancy, Prenatal Exposure Delayed Effects, Prospective Studies, Tandem Mass Spectrometry, Birth size, Per- and polyfluoroalkyl substances, PFAS, Prenatal exposure, Offspring adiposity, Abdominal adiposity
0160-4120
Chen, Ling-Wei
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Ng, Sharon
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Tint, Mya-Thway
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Michael, Navin
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Sadananthan, Suresh Anand
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Ong, Yi Ying
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Yuan, Wen Lun
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Chen, Ze-Ying
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Chen, Chia-Yang
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Godfrey, Keith M.
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Tan, Kok Hian
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Gluckman, Peter D.
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Chong, Yap-Seng
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Eriksson, Johan G.
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Yap, Fabian
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Lee, Yung Seng
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Fortier, Marielle V.
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Velan, Sendhil S.
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Chan, Shiao-Yng
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Chen, Ling-Wei
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Ng, Sharon
cb549f0f-0584-4498-8c49-6023fde1fa87
Tint, Mya-Thway
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Michael, Navin
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Sadananthan, Suresh Anand
41601e35-0034-44a4-b37f-87fc92adfe79
Ong, Yi Ying
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Yuan, Wen Lun
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Chen, Ze-Ying
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Chen, Chia-Yang
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Godfrey, Keith M.
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Tan, Kok Hian
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Gluckman, Peter D.
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Chong, Yap-Seng
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Eriksson, Johan G.
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Yap, Fabian
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Lee, Yung Seng
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Fortier, Marielle V.
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Velan, Sendhil S.
20621485-91f4-4cac-84f2-b39f51e80e45
Chan, Shiao-Yng
3c9d8970-2cc4-430a-86a7-96f6029a5293

Chen, Ling-Wei, Ng, Sharon, Tint, Mya-Thway, Michael, Navin, Sadananthan, Suresh Anand, Ong, Yi Ying, Yuan, Wen Lun, Chen, Ze-Ying, Chen, Chia-Yang, Godfrey, Keith M., Tan, Kok Hian, Gluckman, Peter D., Chong, Yap-Seng, Eriksson, Johan G., Yap, Fabian, Lee, Yung Seng, Fortier, Marielle V., Velan, Sendhil S. and Chan, Shiao-Yng (2024) Associations of cord plasma per- and polyfluoroakyl substances (PFAS) with neonatal and child body composition and adiposity: the GUSTO study. Environment International, 183, [108340]. (doi:10.1016/j.envint.2023.108340).

Record type: Article

Abstract

Background: the influence of prenatal exposure to per- and poly- fluoroalkyl substances (PFAS) on birth size and offspring adiposity is unclear, especially for the newer, shorter-chained replacement PFAS. 

Methods: in the GUSTO multi-ethnic Singaporean mother-offspring cohort, 12 PFAS were measured in 783 cord plasma samples using ultra-performance-liquid chromatography-tandem-mass-spectrometer (UPLC-MS/MS). Outcomes included offspring anthropometry, other indicators of body composition/metabolic health, and MRI-derived abdominal adiposity (subset) at birth and 6 years of age. PFAS were modeled individually, in categories of long-chain and short-chain PFAS, and as scores of three principal components (PC) derived using PC analysis (PC1, PC2, and PC3 reflect predominant exposure patterns to “very-long-PFAS”, “long-PFAS”, and “short-PFAS”, respectively). Associations with outcomes were assessed using multivariable linear regressions, adjusted for important covariates such as maternal sociodemographic and lifestyle factors. 

Results: overall, cord PFAS levels showed either no or positive associations (mostly for long-chain PFAS) with birth weight, length and head circumference. In general, PFAS were associated with higher neonatal abdominal adiposity, driven by shorter-chain PFAS. Perfluoroheptanoic acid (PFHpA) was associated with higher volumes of superficial subcutaneous adipose tissue (sSAT) (3.75 [1.13, 6.37] mL per SD increase in PFAS) and internal adipose tissue (IAT) (1.39 [0.41, 2.38] mL). Higher levels of perfluorobutanesulfonic acid (PFBS), short-chain PFAS, and PC3 were associated with higher IAT volume (β range 1.22–1.41 mL/SD, all P < 0.02), especially in girls. Higher PC3 score was additionally associated with higher sSAT (3.12 [0.45, 5.80] mL) volume. At age 6 years, most observed associations did not persist. No consistent associations were observed between PFAS and whole-body adiposity measures. 

Conclusions: fetal exposure to emerging short-chain PFAS was associated with higher abdominal adiposity at birth but not at age 6 years. Further research is needed to replicate the findings and to determine if these effects may reappear beyond early childhood. Population exposure to newer PFAS and consequent health impact must be monitored.

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Accepted/In Press date: 20 November 2024
e-pub ahead of print date: 22 November 2024
Published date: 3 December 2024
Additional Information: For the purpose of Open Access, the author has applied a Creative Commons Attribution (CC BY) licence to any Author Accepted Manuscript version arising from this submission.
Keywords: Adiposity, Alkanesulfonic Acids, Body Composition, Child, Child, Preschool, Chromatography, Liquid, Environmental Pollutants, Female, Fluorocarbons, Humans, Infant, Newborn, Obesity, Obesity, Abdominal, Pregnancy, Prenatal Exposure Delayed Effects, Prospective Studies, Tandem Mass Spectrometry, Birth size, Per- and polyfluoroalkyl substances, PFAS, Prenatal exposure, Offspring adiposity, Abdominal adiposity

Identifiers

Local EPrints ID: 493606
URI: http://eprints.soton.ac.uk/id/eprint/493606
ISSN: 0160-4120
PURE UUID: e99fc79b-0827-4125-8fe7-fa775c3c5afb
ORCID for Keith M. Godfrey: ORCID iD orcid.org/0000-0002-4643-0618

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Date deposited: 09 Sep 2024 16:41
Last modified: 10 Sep 2024 01:33

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Contributors

Author: Ling-Wei Chen
Author: Sharon Ng
Author: Mya-Thway Tint
Author: Navin Michael
Author: Suresh Anand Sadananthan
Author: Yi Ying Ong
Author: Wen Lun Yuan
Author: Ze-Ying Chen
Author: Chia-Yang Chen
Author: Kok Hian Tan
Author: Peter D. Gluckman
Author: Yap-Seng Chong
Author: Johan G. Eriksson
Author: Fabian Yap
Author: Yung Seng Lee
Author: Marielle V. Fortier
Author: Sendhil S. Velan
Author: Shiao-Yng Chan

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