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Effects of a DC offset on an electrothermal microparticle trap assembled with an AC electric field

Effects of a DC offset on an electrothermal microparticle trap assembled with an AC electric field
Effects of a DC offset on an electrothermal microparticle trap assembled with an AC electric field
Micro and nano-scale colloidal particles can be rapidly assembled at electrode-electrolyte interfaces in highly organized structures. These particles aggregate through various forces which are, among others, chemical, electrical, and thermal in nature. Patterning biological cells in such structures has high impact applications but it remains a challenge due to their limited viability under said manipulation forces. Rapid electrokinetic patterning (REP) uses AC electrothermal micro-vortices to aggregate both synthetic particles and biological cells. In this work, we explore the effects of a DC offset on a REP trap performance in bio-relevant isotonic medium. REP traps were characterized by measuring the inter-particle distance under different DC offsets, using a Delaunay triangulation. The inter-particle distance was measured in a steady-state trap followed by the disassembly of the aggregate as the REP vortex was turned off. DC offset enhanced the trapping performance for micro-particles suspended in a sugar-based isotonic medium. It was observed that an increasingly negative DC offset increased the steady-state inter-particle distance and reduced the rate of disassembly. However, no such trend was found with positive DC offsets. Changing the offset in small steps (<500 mV) affected only the inter-particle distance whereas, larger steps significantly affected the trap stability and size.
Colloidal self-assembly, Electrokinetics, Micro-particle manipulation, Optofluidic, Rapid electrokinetic patterning
0927-7757
Gupta, Kshitiz
726543ab-6767-46cb-89aa-db4ef808dfb7
Green, Nicolas G.
d9b47269-c426-41fd-a41d-5f4579faa581
Wereley, Steven T
b80225dd-e66c-4d34-9317-fcaf48e94677
Gupta, Kshitiz
726543ab-6767-46cb-89aa-db4ef808dfb7
Green, Nicolas G.
d9b47269-c426-41fd-a41d-5f4579faa581
Wereley, Steven T
b80225dd-e66c-4d34-9317-fcaf48e94677

Gupta, Kshitiz, Green, Nicolas G. and Wereley, Steven T (2025) Effects of a DC offset on an electrothermal microparticle trap assembled with an AC electric field. Colloids and Surfaces A: Physicochemical and Engineering Aspects, 705 (1), [135621]. (doi:10.1016/j.colsurfa.2024.135621).

Record type: Article

Abstract

Micro and nano-scale colloidal particles can be rapidly assembled at electrode-electrolyte interfaces in highly organized structures. These particles aggregate through various forces which are, among others, chemical, electrical, and thermal in nature. Patterning biological cells in such structures has high impact applications but it remains a challenge due to their limited viability under said manipulation forces. Rapid electrokinetic patterning (REP) uses AC electrothermal micro-vortices to aggregate both synthetic particles and biological cells. In this work, we explore the effects of a DC offset on a REP trap performance in bio-relevant isotonic medium. REP traps were characterized by measuring the inter-particle distance under different DC offsets, using a Delaunay triangulation. The inter-particle distance was measured in a steady-state trap followed by the disassembly of the aggregate as the REP vortex was turned off. DC offset enhanced the trapping performance for micro-particles suspended in a sugar-based isotonic medium. It was observed that an increasingly negative DC offset increased the steady-state inter-particle distance and reduced the rate of disassembly. However, no such trend was found with positive DC offsets. Changing the offset in small steps (<500 mV) affected only the inter-particle distance whereas, larger steps significantly affected the trap stability and size.

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Effects of DC offset on REP - Version of Record
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More information

Accepted/In Press date: 20 October 2024
e-pub ahead of print date: 22 October 2024
Published date: 20 January 2025
Additional Information: Publisher Copyright: © 2024 Elsevier B.V.
Keywords: Colloidal self-assembly, Electrokinetics, Micro-particle manipulation, Optofluidic, Rapid electrokinetic patterning

Identifiers

Local EPrints ID: 495887
URI: http://eprints.soton.ac.uk/id/eprint/495887
ISSN: 0927-7757
PURE UUID: ee21b340-3bb9-4a06-a353-b6575ffcd646
ORCID for Nicolas G. Green: ORCID iD orcid.org/0000-0001-9230-4455

Catalogue record

Date deposited: 26 Nov 2024 17:48
Last modified: 27 Nov 2024 02:39

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Contributors

Author: Kshitiz Gupta
Author: Nicolas G. Green ORCID iD
Author: Steven T Wereley

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