Quantitative analysis of aligned molecule photoelectron angular distributions
Quantitative analysis of aligned molecule photoelectron angular distributions
Molecular frame photoelectron angular distributions (MFPADs) provide the full available detail of the photoionization process. Careful analysis of the evolving photoelectron angular distribution during the coherent rotation of a nonadiabatically aligned sample of molecules allows the detail which is smoothed out by orientational averaging in the laboratory frame to be resolved. Here we exploit a high flux monochromated HHG lightsource to provide single-photon photoelectron angular distributions of field-free aligned molecules. Our measurements are sensitive to alignment frame variations in even
Woodhouse, Jo
94d6c235-3e1e-44bc-8379-525862fd382c
Thompson, James O.F.
2576003c-596b-4dd0-b024-f965ff120f8a
Benda, Jakub
9d795706-a14e-40a6-ae56-21136224f4d9
Minns, Russell
85280db4-c5a6-4a4c-82fe-75693c6a6045
23 January 2025
Woodhouse, Jo
94d6c235-3e1e-44bc-8379-525862fd382c
Thompson, James O.F.
2576003c-596b-4dd0-b024-f965ff120f8a
Benda, Jakub
9d795706-a14e-40a6-ae56-21136224f4d9
Minns, Russell
85280db4-c5a6-4a4c-82fe-75693c6a6045
Woodhouse, Jo, Thompson, James O.F. and Benda, Jakub
,
et al.
(2025)
Quantitative analysis of aligned molecule photoelectron angular distributions.
Physical Review A, 111 (1), [012815].
(doi:10.1103/PhysRevA.111.012815).
Abstract
Molecular frame photoelectron angular distributions (MFPADs) provide the full available detail of the photoionization process. Careful analysis of the evolving photoelectron angular distribution during the coherent rotation of a nonadiabatically aligned sample of molecules allows the detail which is smoothed out by orientational averaging in the laboratory frame to be resolved. Here we exploit a high flux monochromated HHG lightsource to provide single-photon photoelectron angular distributions of field-free aligned molecules. Our measurements are sensitive to alignment frame variations in even
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Quantitative_analysis_of_aligned_molecule_photoelectron_angular_distributions
- Accepted Manuscript
More information
Accepted/In Press date: 16 December 2024
Published date: 23 January 2025
Identifiers
Local EPrints ID: 498435
URI: http://eprints.soton.ac.uk/id/eprint/498435
ISSN: 1050-2947
PURE UUID: 6963de3f-aec3-4867-82d9-b9680fa9e6bf
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Date deposited: 18 Feb 2025 17:41
Last modified: 14 May 2025 01:59
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Contributors
Author:
Jo Woodhouse
Author:
James O.F. Thompson
Author:
Jakub Benda
Corporate Author: et al.
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