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Atmospheric pressure dielectric barrier discharge plasma for in-situ water treatment using a microbubble reactor

Atmospheric pressure dielectric barrier discharge plasma for in-situ water treatment using a microbubble reactor
Atmospheric pressure dielectric barrier discharge plasma for in-situ water treatment using a microbubble reactor
Non-thermal plasma has been an emerging technology for water treatment for decades. In this study, we have designed and fabricated a bubbling plasma batch reactor using an atmospheric pressure dielectric barrier discharge with a hydrophobic porous membrane. The reactor performance is assessed for purifying synthetic contaminated water samples containing chemical contaminant sulfamethoxazole (SMX), a widely used antibiotic, and biological contaminant E. coli K12. The SMX decontamination tests indicate that the degradation process is not first-order and the reaction rate dwindle with increasing initial concentration. The yield at 50% removal achieves its highest value of 8.12 g/kWh for 50 mg/L SMX sample. For inactivation of E. coli K12 tests, the inactivation process is also not first-order, and the pathogen is completely inactivated for 102 CFU/mL and 104 CFU/mL cases after 10 min and 45 min of plasma treatment, respectively. For the 108 CFU/mL sample, a 5-log reduction is achieved after 60 min of treatment. The developed plasma reactor can achieve fast deployment in point of use, low cost for manufacturing, and simple for maintenance. Moreover, it can be used for in-situ water purification in future long duration crewe
Dielectric barrier discharge, E. coli K12 inactivation, In-situ resource utilization (ISRU), Non-thermal plasma, Sulfamethoxazole degradation
0301-4797
Tang, Xin
8decf9ff-c473-4406-a917-c68766216e5b
Ferraz Júnior, Antônio D.N.
f3af3d30-a40d-48ce-95a4-44190a5efc9e
Karu, Kersti
bf693df4-7839-4c9a-8c62-b454e14c7344
Campos, Luiza C.
c5a66b11-970b-4f6f-88a9-0aadf178b06d
Kim, Minkwan
18ed9a6f-484f-4a7c-bf24-b630938c1acc
Tang, Xin
8decf9ff-c473-4406-a917-c68766216e5b
Ferraz Júnior, Antônio D.N.
f3af3d30-a40d-48ce-95a4-44190a5efc9e
Karu, Kersti
bf693df4-7839-4c9a-8c62-b454e14c7344
Campos, Luiza C.
c5a66b11-970b-4f6f-88a9-0aadf178b06d
Kim, Minkwan
18ed9a6f-484f-4a7c-bf24-b630938c1acc

Tang, Xin, Ferraz Júnior, Antônio D.N., Karu, Kersti, Campos, Luiza C. and Kim, Minkwan (2024) Atmospheric pressure dielectric barrier discharge plasma for in-situ water treatment using a microbubble reactor. Journal of Environmental Management, 370, [122574]. (doi:10.1016/j.jenvman.2024.122574).

Record type: Article

Abstract

Non-thermal plasma has been an emerging technology for water treatment for decades. In this study, we have designed and fabricated a bubbling plasma batch reactor using an atmospheric pressure dielectric barrier discharge with a hydrophobic porous membrane. The reactor performance is assessed for purifying synthetic contaminated water samples containing chemical contaminant sulfamethoxazole (SMX), a widely used antibiotic, and biological contaminant E. coli K12. The SMX decontamination tests indicate that the degradation process is not first-order and the reaction rate dwindle with increasing initial concentration. The yield at 50% removal achieves its highest value of 8.12 g/kWh for 50 mg/L SMX sample. For inactivation of E. coli K12 tests, the inactivation process is also not first-order, and the pathogen is completely inactivated for 102 CFU/mL and 104 CFU/mL cases after 10 min and 45 min of plasma treatment, respectively. For the 108 CFU/mL sample, a 5-log reduction is achieved after 60 min of treatment. The developed plasma reactor can achieve fast deployment in point of use, low cost for manufacturing, and simple for maintenance. Moreover, it can be used for in-situ water purification in future long duration crewe

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Accepted/In Press date: 16 September 2024
e-pub ahead of print date: 24 September 2024
Published date: 24 December 2024
Keywords: Dielectric barrier discharge, E. coli K12 inactivation, In-situ resource utilization (ISRU), Non-thermal plasma, Sulfamethoxazole degradation

Identifiers

Local EPrints ID: 498621
URI: http://eprints.soton.ac.uk/id/eprint/498621
ISSN: 0301-4797
PURE UUID: cab6d805-2a25-495d-9e18-661633b1d5c2
ORCID for Minkwan Kim: ORCID iD orcid.org/0000-0002-6192-312X

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Date deposited: 24 Feb 2025 17:42
Last modified: 28 Feb 2025 02:48

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Contributors

Author: Xin Tang
Author: Antônio D.N. Ferraz Júnior
Author: Kersti Karu
Author: Luiza C. Campos
Author: Minkwan Kim ORCID iD

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