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Hyperuniform designs for enhanced light trapping in ultrathin single and tandem solar cells (Conference Presentation)

Hyperuniform designs for enhanced light trapping in ultrathin single and tandem solar cells (Conference Presentation)
Hyperuniform designs for enhanced light trapping in ultrathin single and tandem solar cells (Conference Presentation)

Introducing thin, light-weight and high efficiency photovoltaics will make solar cells more suitable to be integrated in urban landscapes or even small gadgets and would largely contribute to solving the global warming threat that we are facing today. Stacking of solar cells with different characteristic bandgaps is the most common strategy to surpass the Shockley-Queisser efficiency limit, but such tandem devices are typically heavy weight, rigid and costly. Thinning down of absorber materials is a good strategy to overcome these restrictions. However, nano- and micro-meter thicknesses come down to the expense of light absorption. An effective approach to tackle the absorption problem in thin materials is nanopatterning the absorbing layer. In this work we introduce hyperuniform designs as an effective way to control scattered light into particular range of angles (revealed as a ring in k-space of the reflected/transmitted light), with the aim to efficiently trap light in μm-thick Silicon (Si) cells. We first consider the –theoretical and experimental- case of a single Si solar cell, and thanks to an optimization algorithm, we show the highest light absorption in 1 μm-thick Si film to date. We also compare different designs for best anti-reflection effect on top of light trapping and characterize the increased absorption in photoelectrochemical devices. Second, we incorporate a similar light trapping strategy in a tandem solar cell, by using a periodic GaAs nanowire array as a top cell. We introduce two waveguiding effects in GaAs NW-Si thin film architectures to explain the 4-fold light absorption in the Si ultrathin bottom cell for tailored geometries of the NW array. These results represent significant light trapping scheme that is obtained “for free” when using a nanostructured top cell.
Tavakoli, Nasim
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Spalding, Richard J.
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Gkantzounis, Georgios
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Wan, Chenglong
1dc3bd51-08da-48de-9358-7bddb0d10c73
Röhrich, Ruslan
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Kontoleta, Evgenia
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Florescu, Marian
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Sapienza, Riccardo
dcecc61d-0d12-4cf1-aa98-a3cd940fe0ae
Koenderink, Femius
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Alarcon-Llado, Esther
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Goldschmidt, Jan Christoph
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Sprafke, Alexander N.
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Pandraud, Gregory
b363619e-1fed-48c5-9978-9e6f9bd90c35
Tavakoli, Nasim
aef866e9-ae4a-4c62-9d2f-d527149909d8
Spalding, Richard J.
005f61d7-a04e-43cb-b7a1-dc56c44989a9
Gkantzounis, Georgios
89ac79fa-7f76-4cf0-97d7-cbd84f02b940
Wan, Chenglong
1dc3bd51-08da-48de-9358-7bddb0d10c73
Röhrich, Ruslan
6151ace8-2fb8-4744-96ab-20f66c6c820c
Kontoleta, Evgenia
64513069-4d2d-4d6b-8758-be9d8033ddce
Florescu, Marian
14b7415d-9dc6-4ebe-a125-289e47648c65
Sapienza, Riccardo
dcecc61d-0d12-4cf1-aa98-a3cd940fe0ae
Koenderink, Femius
50383f64-0021-4c74-a8de-eeb4041956cf
Alarcon-Llado, Esther
7bbc03c8-f430-4fa3-8fe6-593a30d92799
Goldschmidt, Jan Christoph
23015c7e-c107-4ab9-9d8a-ce65f7557042
Sprafke, Alexander N.
11b5a201-422f-46aa-8439-65a3692fa7d3
Pandraud, Gregory
b363619e-1fed-48c5-9978-9e6f9bd90c35

Tavakoli, Nasim, Spalding, Richard J., Gkantzounis, Georgios, Wan, Chenglong, Röhrich, Ruslan, Kontoleta, Evgenia, Florescu, Marian, Sapienza, Riccardo, Koenderink, Femius and Alarcon-Llado, Esther (2020) Hyperuniform designs for enhanced light trapping in ultrathin single and tandem solar cells (Conference Presentation). Goldschmidt, Jan Christoph, Sprafke, Alexander N. and Pandraud, Gregory (eds.) SPIE Photonics Europe 2020, , Strasbourg, France. 29 Mar - 02 Apr 2020. (doi:10.1117/12.2554441).

Record type: Conference or Workshop Item (Paper)

Abstract


Introducing thin, light-weight and high efficiency photovoltaics will make solar cells more suitable to be integrated in urban landscapes or even small gadgets and would largely contribute to solving the global warming threat that we are facing today. Stacking of solar cells with different characteristic bandgaps is the most common strategy to surpass the Shockley-Queisser efficiency limit, but such tandem devices are typically heavy weight, rigid and costly. Thinning down of absorber materials is a good strategy to overcome these restrictions. However, nano- and micro-meter thicknesses come down to the expense of light absorption. An effective approach to tackle the absorption problem in thin materials is nanopatterning the absorbing layer. In this work we introduce hyperuniform designs as an effective way to control scattered light into particular range of angles (revealed as a ring in k-space of the reflected/transmitted light), with the aim to efficiently trap light in μm-thick Silicon (Si) cells. We first consider the –theoretical and experimental- case of a single Si solar cell, and thanks to an optimization algorithm, we show the highest light absorption in 1 μm-thick Si film to date. We also compare different designs for best anti-reflection effect on top of light trapping and characterize the increased absorption in photoelectrochemical devices. Second, we incorporate a similar light trapping strategy in a tandem solar cell, by using a periodic GaAs nanowire array as a top cell. We introduce two waveguiding effects in GaAs NW-Si thin film architectures to explain the 4-fold light absorption in the Si ultrathin bottom cell for tailored geometries of the NW array. These results represent significant light trapping scheme that is obtained “for free” when using a nanostructured top cell.

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More information

Published date: 1 April 2020
Venue - Dates: SPIE Photonics Europe 2020, , Strasbourg, France, 2020-03-29 - 2020-04-02

Identifiers

Local EPrints ID: 501967
URI: http://eprints.soton.ac.uk/id/eprint/501967
PURE UUID: ccf5f5f9-a7e4-4784-8ae0-53019428836b
ORCID for Marian Florescu: ORCID iD orcid.org/0000-0001-6278-9164

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Date deposited: 12 Jun 2025 17:10
Last modified: 13 Jun 2025 02:15

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Contributors

Author: Nasim Tavakoli
Author: Richard J. Spalding
Author: Georgios Gkantzounis
Author: Chenglong Wan
Author: Ruslan Röhrich
Author: Evgenia Kontoleta
Author: Marian Florescu ORCID iD
Author: Riccardo Sapienza
Author: Femius Koenderink
Author: Esther Alarcon-Llado
Editor: Jan Christoph Goldschmidt
Editor: Alexander N. Sprafke
Editor: Gregory Pandraud

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