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Neutron diffraction and inelastic neutron scattering investigations of the ordered double perovskite Ba2PrIrO6

Neutron diffraction and inelastic neutron scattering investigations of the ordered double perovskite Ba2PrIrO6
Neutron diffraction and inelastic neutron scattering investigations of the ordered double perovskite Ba2PrIrO6
High-resolution neutron-powder diffraction data show that the double perovskite Ba2PrIrO6 is cubic at ambient temperatures in space group Fm m. Below TN=71 K the compound orders antiferromagnetically with magnetic moments of 0.43(2) ?B at 6 K, on both the Pr4+ and the Ir4+ sites, oriented along the cubic a-axis. Inelastic neutron scattering at 105 K reveals a strong peak at 276 meV and a weak transition at 366 meV. The former is consistent with the crystal field splitting of the Pr4+ ground state under the cubic point symmetry, while the latter peak is due to the intermultiplet transition between the ground state and excited state.
0921-4526
543-545
Kockelmann, W.
da5cf7f6-dd23-4909-b567-2b54a7a72930
Adroja, D.T.
8eaa8fab-9acb-420b-af27-918d6fd01a70
Hillier, A.D.
89e88dd9-6b7a-4b1d-a399-99b5bc301e9a
Wakeshima, M.
4ba0553b-c3a4-4e65-bd3e-ef6e2478808c
Izumiyama, Y.
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Hinatsu, Y.
64053305-7e9a-4a6d-bea7-5e36bef34113
Knight, K.S.
e25bb70a-55c5-471c-8c90-079309411d9f
Visser, D.
b06bc338-cebb-48a2-925c-562803ffebf2
Rainford, B.D.
a57f1153-bbba-49a3-bffc-0d96087156a0
Kockelmann, W.
da5cf7f6-dd23-4909-b567-2b54a7a72930
Adroja, D.T.
8eaa8fab-9acb-420b-af27-918d6fd01a70
Hillier, A.D.
89e88dd9-6b7a-4b1d-a399-99b5bc301e9a
Wakeshima, M.
4ba0553b-c3a4-4e65-bd3e-ef6e2478808c
Izumiyama, Y.
64d4f4a9-9445-4841-8dd8-852c9d552934
Hinatsu, Y.
64053305-7e9a-4a6d-bea7-5e36bef34113
Knight, K.S.
e25bb70a-55c5-471c-8c90-079309411d9f
Visser, D.
b06bc338-cebb-48a2-925c-562803ffebf2
Rainford, B.D.
a57f1153-bbba-49a3-bffc-0d96087156a0

Kockelmann, W., Adroja, D.T., Hillier, A.D., Wakeshima, M., Izumiyama, Y., Hinatsu, Y., Knight, K.S., Visser, D. and Rainford, B.D. (2006) Neutron diffraction and inelastic neutron scattering investigations of the ordered double perovskite Ba2PrIrO6. Physica B: Condensed Matter, 378-380, 543-545. (doi:10.1016/j.physb.2006.01.245).

Record type: Article

Abstract

High-resolution neutron-powder diffraction data show that the double perovskite Ba2PrIrO6 is cubic at ambient temperatures in space group Fm m. Below TN=71 K the compound orders antiferromagnetically with magnetic moments of 0.43(2) ?B at 6 K, on both the Pr4+ and the Ir4+ sites, oriented along the cubic a-axis. Inelastic neutron scattering at 105 K reveals a strong peak at 276 meV and a weak transition at 366 meV. The former is consistent with the crystal field splitting of the Pr4+ ground state under the cubic point symmetry, while the latter peak is due to the intermultiplet transition between the ground state and excited state.

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Published date: 2006

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Local EPrints ID: 57400
URI: http://eprints.soton.ac.uk/id/eprint/57400
ISSN: 0921-4526
PURE UUID: 1d89dc8c-496f-493c-89f2-6dfa7f4b039a

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Date deposited: 13 Aug 2008
Last modified: 15 Mar 2024 11:06

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Contributors

Author: W. Kockelmann
Author: D.T. Adroja
Author: A.D. Hillier
Author: M. Wakeshima
Author: Y. Izumiyama
Author: Y. Hinatsu
Author: K.S. Knight
Author: D. Visser
Author: B.D. Rainford

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