Magneto-optical study of defect induced sharp photoluminescence in LaAlO₃ and SrTiO₃

Sarkar, S., Saha, S., Motapothula, M.R., Patra, A., Cao, B.-C., Prakash, S., Cong, C.X., Mathew, S., Ghosh, S., Yu, T. and Venkatesan, T. (2016) Magneto-optical study of defect induced sharp photoluminescence in LaAlO₃ and SrTiO₃. Scientific Reports, 6, [33145]. (doi:10.1038/srep33145).

Abstract

Strongly correlated electronic systems such as Transition Metal Oxides often possess various mid-gap states originating from intrinsic defects in these materials. In this paper, we investigate an extremely sharp Photoluminescence (PL) transition originating from such defect states in two widely used perovskites, LaAlO₃ and SrTiO₃. A detailed study of the PL as a function of temperature and magnetic field has been conducted to understand the behavior and origin of the transition involved. The temperature dependence of the PL peak position for SrTiO₃ is observed to be opposite to that in LaAlO₃. Our results reveal the presence of a spin/orbital character in these transitions which is evident from the splitting of these defect energy levels under a high magnetic field. These PL transitions have the potential for enabling non-contact thermal and field sensors.

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Contributors

Author: S. Sarkar

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