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Self-organization of Ce adatoms on Ag(111): a kinetic Monte Carlo study

Self-organization of Ce adatoms on Ag(111): a kinetic Monte Carlo study
Self-organization of Ce adatoms on Ag(111): a kinetic Monte Carlo study
One of the most fascinating experimental results in fabrication of artificial nanostructures is the creation of the macroscopically ordered superlattice of Ce adatoms on Ag111 F. Silly et al., Phys. Rev. Lett. 92, 016101 2004. Here, performing kinetic Monte Carlo simulations, we study the formation of Ce superlattice at the atomic scale. It is demonstrated that the surface-state mediated long-range interaction between Ce adatoms can lead to their self-assembly into a well ordered structure. The temperature of the substrate and the concentration of Ce adatoms are shown to play a key role in this process.
1550-235X
035421-[5pp]
Negulyaev, N.N.
52430613-d1a8-49d5-b82f-fb1f40fe4058
Stepanyuk, V.S.
d7f13fd7-3617-444a-bc70-6d8f94b4b344
Niebergall, L.
4d35aa16-bc9c-4a9f-88c2-0ef8e515d8cd
Hergert, W.
8faa698d-3cbf-4d08-8c25-53b27000691c
Fangohr, H.
9b7cfab9-d5dc-45dc-947c-2eba5c81a160
Bruno, P.
6727a494-6644-4f3a-88c7-80f3fe718071
Negulyaev, N.N.
52430613-d1a8-49d5-b82f-fb1f40fe4058
Stepanyuk, V.S.
d7f13fd7-3617-444a-bc70-6d8f94b4b344
Niebergall, L.
4d35aa16-bc9c-4a9f-88c2-0ef8e515d8cd
Hergert, W.
8faa698d-3cbf-4d08-8c25-53b27000691c
Fangohr, H.
9b7cfab9-d5dc-45dc-947c-2eba5c81a160
Bruno, P.
6727a494-6644-4f3a-88c7-80f3fe718071

Negulyaev, N.N., Stepanyuk, V.S., Niebergall, L., Hergert, W., Fangohr, H. and Bruno, P. (2006) Self-organization of Ce adatoms on Ag(111): a kinetic Monte Carlo study. Physical Review B, 74 (3), 035421-[5pp]. (doi:10.1103/PhysRevB.74.035421).

Record type: Article

Abstract

One of the most fascinating experimental results in fabrication of artificial nanostructures is the creation of the macroscopically ordered superlattice of Ce adatoms on Ag111 F. Silly et al., Phys. Rev. Lett. 92, 016101 2004. Here, performing kinetic Monte Carlo simulations, we study the formation of Ce superlattice at the atomic scale. It is demonstrated that the surface-state mediated long-range interaction between Ce adatoms can lead to their self-assembly into a well ordered structure. The temperature of the substrate and the concentration of Ce adatoms are shown to play a key role in this process.

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Published date: 18 July 2006

Identifiers

Local EPrints ID: 64959
URI: http://eprints.soton.ac.uk/id/eprint/64959
ISSN: 1550-235X
PURE UUID: d7ab5d0d-73f4-493f-bd0a-2d0220761b99
ORCID for H. Fangohr: ORCID iD orcid.org/0000-0001-5494-7193

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Date deposited: 27 Jan 2009
Last modified: 16 Mar 2024 03:09

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Contributors

Author: N.N. Negulyaev
Author: V.S. Stepanyuk
Author: L. Niebergall
Author: W. Hergert
Author: H. Fangohr ORCID iD
Author: P. Bruno

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