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Synergistic catalysis: enantioselective addition of alkylbenzoxazoles to enals

Synergistic catalysis: enantioselective addition of alkylbenzoxazoles to enals
Synergistic catalysis: enantioselective addition of alkylbenzoxazoles to enals
A novel catalytic enantioselective methodology based on synergistic catalysis is reported. The strategy involves: 1)?the metal-Lewis-acid activation of alkylazaarenes, and 2)?the secondary-amine activation of enals. Consequently, highly functionalized chiral alkylazaarenes were obtained in good yields and with reasonable stereoselectivity
0947-6539
16853-16857
Meazza, Marta
c4665645-8c77-4cfd-aa02-6bcc3341c1aa
Ceban, Victor
2e53f2b7-42ff-4c26-96e9-ef75891af166
Pitak, Mateusz B.
eeb6a00f-2291-4376-830f-d30dfd607ed1
Coles, Simon J.
3116f58b-c30c-48cf-bdd5-397d1c1fecf8
Rios, Ramon
609bedf2-e886-4d62-a676-a32b6f8c1441
Meazza, Marta
c4665645-8c77-4cfd-aa02-6bcc3341c1aa
Ceban, Victor
2e53f2b7-42ff-4c26-96e9-ef75891af166
Pitak, Mateusz B.
eeb6a00f-2291-4376-830f-d30dfd607ed1
Coles, Simon J.
3116f58b-c30c-48cf-bdd5-397d1c1fecf8
Rios, Ramon
609bedf2-e886-4d62-a676-a32b6f8c1441

Meazza, Marta, Ceban, Victor, Pitak, Mateusz B., Coles, Simon J. and Rios, Ramon (2014) Synergistic catalysis: enantioselective addition of alkylbenzoxazoles to enals. Chemistry - A European Journal, 20 (51), 16853-16857. (doi:10.1002/chem.201404565).

Record type: Article

Abstract

A novel catalytic enantioselective methodology based on synergistic catalysis is reported. The strategy involves: 1)?the metal-Lewis-acid activation of alkylazaarenes, and 2)?the secondary-amine activation of enals. Consequently, highly functionalized chiral alkylazaarenes were obtained in good yields and with reasonable stereoselectivity

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e-pub ahead of print date: 28 October 2014
Published date: 15 December 2014
Organisations: Chemistry
Learn more about Chemistry research

Identifiers

Local EPrints ID: 371765
URI: http://eprints.soton.ac.uk/id/eprint/371765
DOI: doi:10.1002/chem.201404565
ISSN: 0947-6539
PURE UUID: f35d1e5c-7488-455e-9914-38d7c59fd1fb
ORCID for Marta Meazza: ORCID iD orcid.org/0000-0003-4382-0626
ORCID for Mateusz B. Pitak: ORCID iD orcid.org/0000-0002-3680-7100
ORCID for Simon J. Coles: ORCID iD orcid.org/0000-0001-8414-9272
ORCID for Ramon Rios: ORCID iD orcid.org/0000-0002-3843-8521

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Date deposited: 09 Jun 2016 11:04
Last modified: 15 Mar 2024 03:01

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Contributors

Author: Marta Meazza ORCID iD
Author: Victor Ceban
Author: Mateusz B. Pitak ORCID iD
Author: Simon J. Coles ORCID iD
Author: Ramon Rios ORCID iD

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