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Dataset in support of the journal article 'Ultra-low thermal conductivity and improved thermoelectric properties of Al-doped ZnO by in-situ O2 plasma treatment'

Dataset in support of the journal article 'Ultra-low thermal conductivity and improved thermoelectric properties of Al-doped ZnO by in-situ O2 plasma treatment'
Dataset in support of the journal article 'Ultra-low thermal conductivity and improved thermoelectric properties of Al-doped ZnO by in-situ O2 plasma treatment'
The thriving of Internet-of-Things and integrated wireless sensor networks has brought an unprecedented demand for sustainable micro-Watt-scale power supplies. Development of high-performing micro-thermoelectric generator (μ-TEG) that can convert waste thermal energy into electricity and provide sustainable micro-Watt-scale power is therefore extremely timely and important. Herein, a significant advance in the development of earth-abundant, nontoxic thermoelectric materials of aluminium-doped zinc oxide (AZO) is presented. Through nanostructure engineering using a novel in situ O2 plasma treatment, AZO films are demonstrated with ultralow thermal conductivity of 0.16 W m-1 K-1 which is the lowest reported in the literature. This nanostructured film yields a power factor of 294 μW m-1K-2 at 563 K and has resulted in a state-of-the-art ZT of 0.11 at room temperature and 0.72 at 563 K for AZO thin films. Furthermore, the fabrication and testing of a prototype lateral μ-TEG are reported based on the AZO thin film which achieves a power output of 1.08 nW with an applied temperature difference of 16.9 °C.
University of Southampton
Sethi, Vikesh
e0c3adf8-b928-46c4-b59f-4428cafe7774
Sun, Kai
b7c648a3-7be8-4613-9d4d-1bf937fb487b
Newbrook, Daniel
8eb26553-e1e2-492d-ad78-ce51a487f31f
Zhang, Tongjun
4a460cd9-f2c8-41db-8008-1cda74895b24
Runacres, Danielle
aae55f94-b99a-4e9f-9d1b-8bcd3f2a93b6
Greenacre, Victoria
c665a38b-0b1a-4671-ac75-bf0679dd1c57
De Groot, Kees
92cd2e02-fcc4-43da-8816-c86f966be90c
Huang, Ruomeng
c6187811-ef2f-4437-8333-595c0d6ac978
Sethi, Vikesh
e0c3adf8-b928-46c4-b59f-4428cafe7774
Sun, Kai
b7c648a3-7be8-4613-9d4d-1bf937fb487b
Newbrook, Daniel
8eb26553-e1e2-492d-ad78-ce51a487f31f
Zhang, Tongjun
4a460cd9-f2c8-41db-8008-1cda74895b24
Runacres, Danielle
aae55f94-b99a-4e9f-9d1b-8bcd3f2a93b6
Greenacre, Victoria
c665a38b-0b1a-4671-ac75-bf0679dd1c57
De Groot, Kees
92cd2e02-fcc4-43da-8816-c86f966be90c
Huang, Ruomeng
c6187811-ef2f-4437-8333-595c0d6ac978

Sethi, Vikesh (2023) Dataset in support of the journal article 'Ultra-low thermal conductivity and improved thermoelectric properties of Al-doped ZnO by in-situ O2 plasma treatment'. University of Southampton doi:10.5258/SOTON/D2674 [Dataset]

Record type: Dataset

Abstract

The thriving of Internet-of-Things and integrated wireless sensor networks has brought an unprecedented demand for sustainable micro-Watt-scale power supplies. Development of high-performing micro-thermoelectric generator (μ-TEG) that can convert waste thermal energy into electricity and provide sustainable micro-Watt-scale power is therefore extremely timely and important. Herein, a significant advance in the development of earth-abundant, nontoxic thermoelectric materials of aluminium-doped zinc oxide (AZO) is presented. Through nanostructure engineering using a novel in situ O2 plasma treatment, AZO films are demonstrated with ultralow thermal conductivity of 0.16 W m-1 K-1 which is the lowest reported in the literature. This nanostructured film yields a power factor of 294 μW m-1K-2 at 563 K and has resulted in a state-of-the-art ZT of 0.11 at room temperature and 0.72 at 563 K for AZO thin films. Furthermore, the fabrication and testing of a prototype lateral μ-TEG are reported based on the AZO thin film which achieves a power output of 1.08 nW with an applied temperature difference of 16.9 °C.

Spreadsheet
AZO_Paper_Data.xlsx - Dataset
Available under License Creative Commons Attribution.
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Text
README.txt - Dataset
Available under License Creative Commons Attribution.
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More information

Published date: 18 July 2023

Identifiers

Local EPrints ID: 479015
URI: http://eprints.soton.ac.uk/id/eprint/479015
PURE UUID: 8f762e52-7ef0-45b1-83de-79753b639357
ORCID for Vikesh Sethi: ORCID iD orcid.org/0009-0002-2711-1889
ORCID for Kai Sun: ORCID iD orcid.org/0000-0001-6807-6253
ORCID for Daniel Newbrook: ORCID iD orcid.org/0000-0002-5047-6168
ORCID for Danielle Runacres: ORCID iD orcid.org/0000-0002-2446-1763
ORCID for Victoria Greenacre: ORCID iD orcid.org/0000-0002-3381-9616
ORCID for Kees De Groot: ORCID iD orcid.org/0000-0002-3850-7101
ORCID for Ruomeng Huang: ORCID iD orcid.org/0000-0003-1185-635X

Catalogue record

Date deposited: 18 Jul 2023 16:35
Last modified: 15 Jun 2024 01:42

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Contributors

Creator: Vikesh Sethi ORCID iD
Contributor: Kai Sun ORCID iD
Contributor: Daniel Newbrook ORCID iD
Contributor: Tongjun Zhang
Contributor: Danielle Runacres ORCID iD
Contributor: Victoria Greenacre ORCID iD
Research team head: Kees De Groot ORCID iD
Research team head: Ruomeng Huang ORCID iD

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