Effects of laser linewidth on coherent antiStokes Raman spectroscopy
Effects of laser linewidth on coherent antiStokes Raman spectroscopy
Expressions for the generated antiStokes spectral density in coherent antiStokes Raman spectroscopy (CARS) are obtained, which take into account the finite linewidths of laser sources and which may be used to analyse observed spectra. Lorentzian and Gaussian laser lineshapes are taken as special cases, which enable further analytic results for single and multiline CARS spectra to be derived. Emphasis is placed on scanning and broadband (multiplex) CARS techniques, and the choice of laser sources discussed from the spectral point of view. As examples of multiline spectra an analytical account of a periodic spectrum is presented and temperature measurement from Q-branch spectra is treated.
625-655
Yuratich, M.A.
80b84a92-aa40-4e03-8c65-993ee5729380
1979
Yuratich, M.A.
80b84a92-aa40-4e03-8c65-993ee5729380
Yuratich, M.A.
(1979)
Effects of laser linewidth on coherent antiStokes Raman spectroscopy.
Molecular Physics, 38 (2), .
(doi:10.1080/00268977900101941).
Abstract
Expressions for the generated antiStokes spectral density in coherent antiStokes Raman spectroscopy (CARS) are obtained, which take into account the finite linewidths of laser sources and which may be used to analyse observed spectra. Lorentzian and Gaussian laser lineshapes are taken as special cases, which enable further analytic results for single and multiline CARS spectra to be derived. Emphasis is placed on scanning and broadband (multiplex) CARS techniques, and the choice of laser sources discussed from the spectral point of view. As examples of multiline spectra an analytical account of a periodic spectrum is presented and temperature measurement from Q-branch spectra is treated.
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Published date: 1979
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Local EPrints ID: 78707
URI: http://eprints.soton.ac.uk/id/eprint/78707
ISSN: 0026-8976
PURE UUID: 3c4ba0b0-d5bc-4d8b-bc2b-79ee98b9a673
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Date deposited: 11 Mar 2010
Last modified: 14 Mar 2024 00:20
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Author:
M.A. Yuratich
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