Effects of laser linewidth on coherent antiStokes Raman spectroscopy

Yuratich, M.A. (1979) Effects of laser linewidth on coherent antiStokes Raman spectroscopy Molecular Physics, 38, (2), pp. 625-655. (doi:10.1080/00268977900101941).


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Expressions for the generated antiStokes spectral density in coherent antiStokes Raman spectroscopy (CARS) are obtained, which take into account the finite linewidths of laser sources and which may be used to analyse observed spectra. Lorentzian and Gaussian laser lineshapes are taken as special cases, which enable further analytic results for single and multiline CARS spectra to be derived. Emphasis is placed on scanning and broadband (multiplex) CARS techniques, and the choice of laser sources discussed from the spectral point of view. As examples of multiline spectra an analytical account of a periodic spectrum is presented and temperature measurement from Q-branch spectra is treated.

Item Type: Article
Digital Object Identifier (DOI): doi:10.1080/00268977900101941
ISSNs: 0026-8976 (print)
Related URLs:
ePrint ID: 78707
Date :
Date Event
Date Deposited: 11 Mar 2010
Last Modified: 18 Apr 2017 20:20
Further Information:Google Scholar
URI: http://eprints.soton.ac.uk/id/eprint/78707

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