Coherent anti-Stokes Raman spectroscopy (CARS) selection rules, depolarization ratios and rotational structure
Coherent anti-Stokes Raman spectroscopy (CARS) selection rules, depolarization ratios and rotational structure
By putting the non-linear susceptibility tensors in irreducible spherical form it is found that orientation averaging, selection rules, and the angular dependence of intensity on field polarizations all follow in a straightforward way. These spherical tensor techniques are used to treat coherent anti-Stokes Raman scattering (CARS) in detail and a comparison is made with conventional Raman scattering. The selection rules for both processes are shown to be the same. The paper concludes with a brief discussion of the rotational structure in CARS.
671-682
Yuratich, M.A.
80b84a92-aa40-4e03-8c65-993ee5729380
Hanna, D.C.
3da5a5b4-71c2-4441-bb67-21f0d28a187d
March 1977
Yuratich, M.A.
80b84a92-aa40-4e03-8c65-993ee5729380
Hanna, D.C.
3da5a5b4-71c2-4441-bb67-21f0d28a187d
Yuratich, M.A. and Hanna, D.C.
(1977)
Coherent anti-Stokes Raman spectroscopy (CARS) selection rules, depolarization ratios and rotational structure.
Molecular Physics, 33 (3), .
(doi:10.1080/00268977700100631).
Abstract
By putting the non-linear susceptibility tensors in irreducible spherical form it is found that orientation averaging, selection rules, and the angular dependence of intensity on field polarizations all follow in a straightforward way. These spherical tensor techniques are used to treat coherent anti-Stokes Raman scattering (CARS) in detail and a comparison is made with conventional Raman scattering. The selection rules for both processes are shown to be the same. The paper concludes with a brief discussion of the rotational structure in CARS.
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Published date: March 1977
Identifiers
Local EPrints ID: 78788
URI: http://eprints.soton.ac.uk/id/eprint/78788
ISSN: 0026-8976
PURE UUID: 79a9c75e-c190-4a1e-8c9e-451dfc41c507
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Date deposited: 11 Mar 2010
Last modified: 14 Mar 2024 00:22
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Author:
M.A. Yuratich
Author:
D.C. Hanna
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