Coherent anti-Stokes Raman spectroscopy (CARS) selection rules, depolarization ratios and rotational structure


Yuratich, M.A. and Hanna, D.C. (1977) Coherent anti-Stokes Raman spectroscopy (CARS) selection rules, depolarization ratios and rotational structure Molecular Physics, 33, (3), pp. 671-682. (doi:10.1080/00268977700100631).

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Description/Abstract

By putting the non-linear susceptibility tensors in irreducible spherical form it is found that orientation averaging, selection rules, and the angular dependence of intensity on field polarizations all follow in a straightforward way. These spherical tensor techniques are used to treat coherent anti-Stokes Raman scattering (CARS) in detail and a comparison is made with conventional Raman scattering. The selection rules for both processes are shown to be the same. The paper concludes with a brief discussion of the rotational structure in CARS.

Item Type: Article
Digital Object Identifier (DOI): doi:10.1080/00268977700100631
ISSNs: 0026-8976 (print)
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ePrint ID: 78788
Date :
Date Event
March 1977Published
Date Deposited: 11 Mar 2010
Last Modified: 18 Apr 2017 20:20
Further Information:Google Scholar
URI: http://eprints.soton.ac.uk/id/eprint/78788

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